Research output: Contribution to journal › Article › peer-review
Self-Equilibration of the Diameter of Ga-Catalyzed GaAs Nanowires. / Dubrovskii, V. G.; Xu, T.; Álvarez, A. Díaz; Plissard, S. R.; Caroff, P.; Glas, F.; Grandidier, B.
In: Nano Letters, Vol. 15, No. 8, 12.08.2015, p. 5580-5584.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Self-Equilibration of the Diameter of Ga-Catalyzed GaAs Nanowires
AU - Dubrovskii, V. G.
AU - Xu, T.
AU - Álvarez, A. Díaz
AU - Plissard, S. R.
AU - Caroff, P.
AU - Glas, F.
AU - Grandidier, B.
PY - 2015/8/12
Y1 - 2015/8/12
N2 - Designing strategies to reach monodispersity in fabrication of semiconductor nanowire ensembles is essential for numerous applications. When Ga-catalyzed GaAs nanowire arrays are grown by molecular beam epitaxy with help of droplet-engineering, we observe a significant narrowing of the diameter distribution of the final nanowire array with respect to the size distribution of the initial Ga droplets. Considering that the droplet serves as a nonequilibrium reservoir of a group III metal, we develop a model that demonstrates a self-equilibration effect on the droplet size in self-catalyzed III-V nanowires. This effect leads to arrays of nanowires with a high degree of uniformity regardless of the initial conditions, while the stationary diameter can be further finely tuned by varying the spacing of the array pitch on patterned Si substrates.
AB - Designing strategies to reach monodispersity in fabrication of semiconductor nanowire ensembles is essential for numerous applications. When Ga-catalyzed GaAs nanowire arrays are grown by molecular beam epitaxy with help of droplet-engineering, we observe a significant narrowing of the diameter distribution of the final nanowire array with respect to the size distribution of the initial Ga droplets. Considering that the droplet serves as a nonequilibrium reservoir of a group III metal, we develop a model that demonstrates a self-equilibration effect on the droplet size in self-catalyzed III-V nanowires. This effect leads to arrays of nanowires with a high degree of uniformity regardless of the initial conditions, while the stationary diameter can be further finely tuned by varying the spacing of the array pitch on patterned Si substrates.
KW - focusing effect
KW - growth kinetics
KW - III-V nanowires
KW - self-catalyzed growth
KW - silicon integration
KW - size distribution
UR - http://www.scopus.com/inward/record.url?scp=84939244408&partnerID=8YFLogxK
U2 - 10.1021/acs.nanolett.5b02226
DO - 10.1021/acs.nanolett.5b02226
M3 - Article
AN - SCOPUS:84939244408
VL - 15
SP - 5580
EP - 5584
JO - Nano Letters
JF - Nano Letters
SN - 1530-6984
IS - 8
ER -
ID: 107073070