Ссылки

DOI

  • Oxana V. Karimova
  • N. N. Eremin
  • A. A. Mezhueva
  • N. S. Uporova
  • A. A. Zolotarev
  • D. A. Chareev
The phase transition in the structure of the PdBi2 compound was studied using high-temperature in-situ methods (differential thermal analysis, high-temperature single-crystal X-ray diffraction). The structures of PdBi2 polymorphic modifications were refined at temperatures of 300, 373, 473, 573 and 637 K based on the high-temperature single-crystal X-ray diffraction data. A low-temperature modification of α-PdBi2 is monoclinic, space group C2/m (a = 12.726(1)A, b = 4.2605(4)A, c = 5.5668(5)A, β = 102.51(1) °, V = 299.95(5)A3, Z = 2). It is stable in the temperature range from 300K (27 °C) to 573K (300 °С) and is corresponding to the mineral froodite. A high-temperature modification of β-PdBi2 was fixed at the temperature 673K (400 °C). The phase β-PdBi2 is structural analogue of the mineral urvancevite: it’s tetragonal, space group I4/mmm (a = 3.3876(3) A, c = 13.092(2) A, V = 150.24(4) A3, Z = 1). The phase transition refers to a type I and is a reconstructive polymorphic transformation with a rearrangement of the first coordination sphere.
Язык оригиналаанглийский
Страницы (с-по)3-9
Число страниц7
ЖурналВЕСТНИК МОСКОВСКОГО УНИВЕРСИТЕТА. СЕРИЯ 4: ГЕОЛОГИЯ
Том64
Номер выпуска1
DOI
СостояниеОпубликовано - 1 янв 2025

ID: 135531548