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Time-resolved inner-shell photoelectron spectroscopy : From a bound molecule to an isolated atom. / Brasse, Felix; Goldsztejn, Gildas; Amini, Kasra; Boll, Rebecca; Bari, Sadia; Bomme, Cedric; Brouard, Mark; Burt, Michael; de Miranda, Barbara Cunha; Duesterer, Stefan; Erk, Benjamin; Geleoc, Marie; Geneaux, Romain; Gentleman, Alexander S.; Guillemin, Renaud; Ismail, Iyas; Johnsson, Per; Journel, Loic; Kierspel, Thomas; Kockert, Hansjochen; Kuepper, Jochen; Lablanquie, Pascal; Lahl, Jan; Lee, Jason W. L.; Mackenzie, Stuart R.; Maclot, Sylvain; Manschwetus, Bastian; Mereshchenko, Andrey S.; Mullins, Terence; Olshin, Pavel K.; Palaudoux, Jerome; Patchkovskii, Serguei; Penent, Francis; Piancastelli, Maria Novella; Rompotis, Dimitrios; Ruchon, Thierry; Rudenko, Artem; Savelyev, Evgeny; Schirmel, Nora; Techert, Simone; Travnikova, Oksana; Trippel, Sebastian; Underwood, Jonathan G.; Vallance, Claire; Wiese, Joss; Simon, Marc; Holland, David M. P.; Marchenko, Tatiana; Rouzee, Arnaud; Rolles, Daniel.

In: Physical Review A - Atomic, Molecular, and Optical Physics, Vol. 97, No. 4, 043429, 27.04.2018.

Research output: Contribution to journal › Article › peer-review

Harvard

Brasse, F, Goldsztejn, G, Amini, K, Boll, R, Bari, S, Bomme, C, Brouard, M, Burt, M, de Miranda, BC, Duesterer, S, Erk, B, Geleoc, M, Geneaux, R, Gentleman, AS, Guillemin, R, Ismail, I, Johnsson, P, Journel, L, Kierspel, T, Kockert, H, Kuepper, J, Lablanquie, P, Lahl, J, Lee, JWL, Mackenzie, SR, Maclot, S, Manschwetus, B, Mereshchenko, AS, Mullins, T, Olshin, PK, Palaudoux, J, Patchkovskii, S, Penent, F, Piancastelli, MN, Rompotis, D, Ruchon, T, Rudenko, A, Savelyev, E, Schirmel, N, Techert, S, Travnikova, O, Trippel, S, Underwood, JG, Vallance, C, Wiese, J, Simon, M, Holland, DMP, Marchenko, T, Rouzee, A & Rolles, D 2018, 'Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom', Physical Review A - Atomic, Molecular, and Optical Physics, vol. 97, no. 4, 043429. https://doi.org/10.1103/PhysRevA.97.043429

APA

Brasse, F., Goldsztejn, G., Amini, K., Boll, R., Bari, S., Bomme, C., Brouard, M., Burt, M., de Miranda, B. C., Duesterer, S., Erk, B., Geleoc, M., Geneaux, R., Gentleman, A. S., Guillemin, R., Ismail, I., Johnsson, P., Journel, L., Kierspel, T., ... Rolles, D. (2018). Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom. Physical Review A - Atomic, Molecular, and Optical Physics, 97(4), [043429]. https://doi.org/10.1103/PhysRevA.97.043429

Vancouver

Brasse F, Goldsztejn G, Amini K, Boll R, Bari S, Bomme C et al. Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom. Physical Review A - Atomic, Molecular, and Optical Physics. 2018 Apr 27;97(4). 043429. https://doi.org/10.1103/PhysRevA.97.043429

Author

Brasse, Felix ; Goldsztejn, Gildas ; Amini, Kasra ; Boll, Rebecca ; Bari, Sadia ; Bomme, Cedric ; Brouard, Mark ; Burt, Michael ; de Miranda, Barbara Cunha ; Duesterer, Stefan ; Erk, Benjamin ; Geleoc, Marie ; Geneaux, Romain ; Gentleman, Alexander S. ; Guillemin, Renaud ; Ismail, Iyas ; Johnsson, Per ; Journel, Loic ; Kierspel, Thomas ; Kockert, Hansjochen ; Kuepper, Jochen ; Lablanquie, Pascal ; Lahl, Jan ; Lee, Jason W. L. ; Mackenzie, Stuart R. ; Maclot, Sylvain ; Manschwetus, Bastian ; Mereshchenko, Andrey S. ; Mullins, Terence ; Olshin, Pavel K. ; Palaudoux, Jerome ; Patchkovskii, Serguei ; Penent, Francis ; Piancastelli, Maria Novella ; Rompotis, Dimitrios ; Ruchon, Thierry ; Rudenko, Artem ; Savelyev, Evgeny ; Schirmel, Nora ; Techert, Simone ; Travnikova, Oksana ; Trippel, Sebastian ; Underwood, Jonathan G. ; Vallance, Claire ; Wiese, Joss ; Simon, Marc ; Holland, David M. P. ; Marchenko, Tatiana ; Rouzee, Arnaud ; Rolles, Daniel. / Time-resolved inner-shell photoelectron spectroscopy : From a bound molecule to an isolated atom. In: Physical Review A - Atomic, Molecular, and Optical Physics. 2018 ; Vol. 97, No. 4.

BibTeX

@article{cac87b5c2bd6460bb77e3871d83e348c,
title = "Time-resolved inner-shell photoelectron spectroscopy: From a bound molecule to an isolated atom",
abstract = "Due to its element and site specificity, inner-shell photoelectron spectroscopy is a widely used technique to probe the chemical structure of matter. Here, we show that time-resolved inner-shell photoelectron spectroscopy can be employed to observe ultrafast chemical reactions and the electronic response to the nuclear motion with high sensitivity. The ultraviolet dissociation of iodomethane (CH3I) is investigated by ionization above the iodine 4d edge, using time-resolved inner-shell photoelectron and photoion spectroscopy. The dynamics observed in the photoelectron spectra appear earlier and are faster than those seen in the iodine fragments. The experimental results are interpreted using crystal-field and spin-orbit configuration interaction calculations, and demonstrate that time-resolved inner-shell photoelectron spectroscopy is a powerful tool to directly track ultrafast structural and electronic transformations in gas-phase molecules.",
keywords = "FREE-ELECTRON LASER, CONICAL INTERSECTIONS, SYNCHROTRON-RADIATION, METHYL-IODIDE, DYNAMICS, PHOTODISSOCIATION, PHOTOIONIZATION, PHOTOABSORPTION, ENERGY, FIELD",
author = "Felix Brasse and Gildas Goldsztejn and Kasra Amini and Rebecca Boll and Sadia Bari and Cedric Bomme and Mark Brouard and Michael Burt and {de Miranda}, {Barbara Cunha} and Stefan Duesterer and Benjamin Erk and Marie Geleoc and Romain Geneaux and Gentleman, {Alexander S.} and Renaud Guillemin and Iyas Ismail and Per Johnsson and Loic Journel and Thomas Kierspel and Hansjochen Kockert and Jochen Kuepper and Pascal Lablanquie and Jan Lahl and Lee, {Jason W. L.} and Mackenzie, {Stuart R.} and Sylvain Maclot and Bastian Manschwetus and Mereshchenko, {Andrey S.} and Terence Mullins and Olshin, {Pavel K.} and Jerome Palaudoux and Serguei Patchkovskii and Francis Penent and Piancastelli, {Maria Novella} and Dimitrios Rompotis and Thierry Ruchon and Artem Rudenko and Evgeny Savelyev and Nora Schirmel and Simone Techert and Oksana Travnikova and Sebastian Trippel and Underwood, {Jonathan G.} and Claire Vallance and Joss Wiese and Marc Simon and Holland, {David M. P.} and Tatiana Marchenko and Arnaud Rouzee and Daniel Rolles",
year = "2018",
month = apr,
day = "27",
doi = "10.1103/PhysRevA.97.043429",
language = "Английский",
volume = "97",
journal = "Physical Review A - Atomic, Molecular, and Optical Physics",
issn = "1050-2947",
publisher = "American Physical Society",
number = "4",

}

RIS

TY - JOUR

T1 - Time-resolved inner-shell photoelectron spectroscopy

T2 - From a bound molecule to an isolated atom

AU - Brasse, Felix

AU - Goldsztejn, Gildas

AU - Amini, Kasra

AU - Boll, Rebecca

AU - Bari, Sadia

AU - Bomme, Cedric

AU - Brouard, Mark

AU - Burt, Michael

AU - de Miranda, Barbara Cunha

AU - Duesterer, Stefan

AU - Erk, Benjamin

AU - Geleoc, Marie

AU - Geneaux, Romain

AU - Gentleman, Alexander S.

AU - Guillemin, Renaud

AU - Ismail, Iyas

AU - Johnsson, Per

AU - Journel, Loic

AU - Kierspel, Thomas

AU - Kockert, Hansjochen

AU - Kuepper, Jochen

AU - Lablanquie, Pascal

AU - Lahl, Jan

AU - Lee, Jason W. L.

AU - Mackenzie, Stuart R.

AU - Maclot, Sylvain

AU - Manschwetus, Bastian

AU - Mereshchenko, Andrey S.

AU - Mullins, Terence

AU - Olshin, Pavel K.

AU - Palaudoux, Jerome

AU - Patchkovskii, Serguei

AU - Penent, Francis

AU - Piancastelli, Maria Novella

AU - Rompotis, Dimitrios

AU - Ruchon, Thierry

AU - Rudenko, Artem

AU - Savelyev, Evgeny

AU - Schirmel, Nora

AU - Techert, Simone

AU - Travnikova, Oksana

AU - Trippel, Sebastian

AU - Underwood, Jonathan G.

AU - Vallance, Claire

AU - Wiese, Joss

AU - Simon, Marc

AU - Holland, David M. P.

AU - Marchenko, Tatiana

AU - Rouzee, Arnaud

AU - Rolles, Daniel

PY - 2018/4/27

Y1 - 2018/4/27

N2 - Due to its element and site specificity, inner-shell photoelectron spectroscopy is a widely used technique to probe the chemical structure of matter. Here, we show that time-resolved inner-shell photoelectron spectroscopy can be employed to observe ultrafast chemical reactions and the electronic response to the nuclear motion with high sensitivity. The ultraviolet dissociation of iodomethane (CH3I) is investigated by ionization above the iodine 4d edge, using time-resolved inner-shell photoelectron and photoion spectroscopy. The dynamics observed in the photoelectron spectra appear earlier and are faster than those seen in the iodine fragments. The experimental results are interpreted using crystal-field and spin-orbit configuration interaction calculations, and demonstrate that time-resolved inner-shell photoelectron spectroscopy is a powerful tool to directly track ultrafast structural and electronic transformations in gas-phase molecules.

AB - Due to its element and site specificity, inner-shell photoelectron spectroscopy is a widely used technique to probe the chemical structure of matter. Here, we show that time-resolved inner-shell photoelectron spectroscopy can be employed to observe ultrafast chemical reactions and the electronic response to the nuclear motion with high sensitivity. The ultraviolet dissociation of iodomethane (CH3I) is investigated by ionization above the iodine 4d edge, using time-resolved inner-shell photoelectron and photoion spectroscopy. The dynamics observed in the photoelectron spectra appear earlier and are faster than those seen in the iodine fragments. The experimental results are interpreted using crystal-field and spin-orbit configuration interaction calculations, and demonstrate that time-resolved inner-shell photoelectron spectroscopy is a powerful tool to directly track ultrafast structural and electronic transformations in gas-phase molecules.

KW - FREE-ELECTRON LASER

KW - CONICAL INTERSECTIONS

KW - SYNCHROTRON-RADIATION

KW - METHYL-IODIDE

KW - DYNAMICS

KW - PHOTODISSOCIATION

KW - PHOTOIONIZATION

KW - PHOTOABSORPTION

KW - ENERGY

KW - FIELD

UR - http://www.mendeley.com/research/timeresolved-innershell-photoelectron-spectroscopy-bound-molecule-isolated-atom

U2 - 10.1103/PhysRevA.97.043429

DO - 10.1103/PhysRevA.97.043429

M3 - статья

VL - 97

JO - Physical Review A - Atomic, Molecular, and Optical Physics

JF - Physical Review A - Atomic, Molecular, and Optical Physics

SN - 1050-2947

IS - 4

M1 - 043429

ER -

ID: 27324932