Research output: Contribution to journal › Article › peer-review
The successive ionization potentials (IPs) and electron affinities (EAs) for superheavy elements with 111≤Z≤114, namely, Rg, Cn, Nh, and Fl, are reexamined using the relativistic Fock-space coupled-cluster method with nonperturbative single (S), double (D), and triple (T) cluster amplitudes (FS-CCSDT). For most of the considered quantities, the triple-amplitude contributions turn out to be important. The Breit and frequency-dependent Breit corrections are evaluated by means of the configuration-interaction method. The quantum-electrodynamics corrections to the IPs and EAs are taken into account within the model-QED-operator approach. The obtained results are within 0.10 eV uncertainty.
Original language | English |
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Article number | 062805 |
Pages (from-to) | 062805 |
Journal | Physical Review A - Atomic, Molecular, and Optical Physics |
Volume | 105 |
Issue number | 6 |
DOIs | |
State | Published - 8 Jun 2022 |
ID: 95736180