DOI

In this paper, we report the results of experimental study of electron transport mechanisms in ferroelectric BaTiO 3 ultrathin epitaxial films in a broad temperature range. For this purpose ferroelectric tunnel junctions based on STO/LSMO/BTO/Au structures were fabricated with different thicknesses of ferroelectric films (from 3 to 12 nm). Ferroelectric and electrical properties of heterostructures were measured at temperatures ranging from 40 K to 300 K. Based on experimental results, we find that prevailing transport mechanisms in BaTiO 3 epitaxial thin film is determined by the film thickness. Below the certain thickness of the BaTiO 3 film, a dominant contribution in the current through the structure is due to elastic tunneling. Increasing the thickness of the ferroelectric film leads to an impact from inelastic tunneling, mainly due to an interaction with traps caused by cation and anion vacancies in oxide sub-lattices. We suppose that the specificity of transport mechanisms in BaTiO 3 ultrathin films is defined by the ratio of film thickness and the mean free path of injected electrons, along with repolarization processes synchronized with the ferroelectric coercive field. The latter point has been confirmed by the results of experimental study in a broad temperature range.

Язык оригиналаанглийский
Номер статьи026427
Число страниц7
ЖурналMaterials Research Express
Том6
Номер выпуска2
DOI
СостояниеОпубликовано - фев 2019

    Предметные области Scopus

  • Электроника, оптика и магнитные материалы
  • Металлы и сплавы
  • Поверхности, слои и пленки
  • Пластик и полимеры
  • Биоматериалы

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