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Influence of State-to-State Vibrational Distributions onTransport Coefficients of a Single Gas. / Kustova, E.V.; Kremer, G.M.

в: AIP Conference Proceedings, Том 1786, 070002, 2016.

Результаты исследований: Научные публикации в периодических изданияхстатьяРецензирование

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@article{312a0fe11217479f8187a9479b5b07a0,
title = "Influence of State-to-State Vibrational Distributions onTransport Coefficients of a Single Gas",
abstract = "In this work the influence of the size of vibrationally and rotationally excited molecules on the collision integrals required for the calculation of state-to-state transport coefficients is discussed. Several diatomic molecules are considered: N2, O2, NO, H2, Cl2. It is shown that whereas the molecular size is not affected by rotational excitation, it strongly depends on the vibrational state. Particular emphasis is given to the shear viscosity and thermal conductivity coefficients calculated in the temperature range 2 500–20 000 K for equilibrium Boltzmann vibrational distributions. It is shown that under conditions of local thermal equilibrium, the effect of vibrational excitation on the shear viscosity and thermal conductivity coefficients are found to be negligible for temperatures below 5 000 K, except for the case of Cl2 molecule where at 5 000 K the effect is about 10% . For T > 10 000 K, the contribution of excited states becomes important and reaches 10–25%.",
author = "E.V. Kustova and G.M. Kremer",
year = "2016",
doi = "10.1063/1.4967578",
language = "English",
volume = "1786",
journal = "AIP Conference Proceedings",
issn = "0094-243X",
publisher = "American Institute of Physics",

}

RIS

TY - JOUR

T1 - Influence of State-to-State Vibrational Distributions onTransport Coefficients of a Single Gas

AU - Kustova, E.V.

AU - Kremer, G.M.

PY - 2016

Y1 - 2016

N2 - In this work the influence of the size of vibrationally and rotationally excited molecules on the collision integrals required for the calculation of state-to-state transport coefficients is discussed. Several diatomic molecules are considered: N2, O2, NO, H2, Cl2. It is shown that whereas the molecular size is not affected by rotational excitation, it strongly depends on the vibrational state. Particular emphasis is given to the shear viscosity and thermal conductivity coefficients calculated in the temperature range 2 500–20 000 K for equilibrium Boltzmann vibrational distributions. It is shown that under conditions of local thermal equilibrium, the effect of vibrational excitation on the shear viscosity and thermal conductivity coefficients are found to be negligible for temperatures below 5 000 K, except for the case of Cl2 molecule where at 5 000 K the effect is about 10% . For T > 10 000 K, the contribution of excited states becomes important and reaches 10–25%.

AB - In this work the influence of the size of vibrationally and rotationally excited molecules on the collision integrals required for the calculation of state-to-state transport coefficients is discussed. Several diatomic molecules are considered: N2, O2, NO, H2, Cl2. It is shown that whereas the molecular size is not affected by rotational excitation, it strongly depends on the vibrational state. Particular emphasis is given to the shear viscosity and thermal conductivity coefficients calculated in the temperature range 2 500–20 000 K for equilibrium Boltzmann vibrational distributions. It is shown that under conditions of local thermal equilibrium, the effect of vibrational excitation on the shear viscosity and thermal conductivity coefficients are found to be negligible for temperatures below 5 000 K, except for the case of Cl2 molecule where at 5 000 K the effect is about 10% . For T > 10 000 K, the contribution of excited states becomes important and reaches 10–25%.

U2 - 10.1063/1.4967578

DO - 10.1063/1.4967578

M3 - Article

VL - 1786

JO - AIP Conference Proceedings

JF - AIP Conference Proceedings

SN - 0094-243X

M1 - 070002

ER -

ID: 7595332