Standard

Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging. / Carnis, Jerome; Kirner, Felizitas; Lapkin, Dmitry; Sturm, Sebastian; Kim, Young Yong; Baburin, Igor A.; Khubbutdinov, Ruslan; Ignatenko, Alexandr; Iashina, Ekaterina; Mistonov, Alexander; Steegemans, Tristan; Wieck, Thomas; Gemming, Thomas; Lubk, Axel; Lazarev, Sergey; Sprung, Michael; Vartanyants, Ivan A.; Sturm, Elena V.

в: Nanoscale, Том 13, № 23, 21.06.2021, стр. 10425-10435.

Результаты исследований: Научные публикации в периодических изданияхстатьяРецензирование

Harvard

Carnis, J, Kirner, F, Lapkin, D, Sturm, S, Kim, YY, Baburin, IA, Khubbutdinov, R, Ignatenko, A, Iashina, E, Mistonov, A, Steegemans, T, Wieck, T, Gemming, T, Lubk, A, Lazarev, S, Sprung, M, Vartanyants, IA & Sturm, EV 2021, 'Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging', Nanoscale, Том. 13, № 23, стр. 10425-10435. https://doi.org/10.1039/d1nr01806j

APA

Carnis, J., Kirner, F., Lapkin, D., Sturm, S., Kim, Y. Y., Baburin, I. A., Khubbutdinov, R., Ignatenko, A., Iashina, E., Mistonov, A., Steegemans, T., Wieck, T., Gemming, T., Lubk, A., Lazarev, S., Sprung, M., Vartanyants, I. A., & Sturm, E. V. (2021). Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging. Nanoscale, 13(23), 10425-10435. https://doi.org/10.1039/d1nr01806j

Vancouver

Carnis J, Kirner F, Lapkin D, Sturm S, Kim YY, Baburin IA и пр. Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging. Nanoscale. 2021 Июнь 21;13(23):10425-10435. https://doi.org/10.1039/d1nr01806j

Author

Carnis, Jerome ; Kirner, Felizitas ; Lapkin, Dmitry ; Sturm, Sebastian ; Kim, Young Yong ; Baburin, Igor A. ; Khubbutdinov, Ruslan ; Ignatenko, Alexandr ; Iashina, Ekaterina ; Mistonov, Alexander ; Steegemans, Tristan ; Wieck, Thomas ; Gemming, Thomas ; Lubk, Axel ; Lazarev, Sergey ; Sprung, Michael ; Vartanyants, Ivan A. ; Sturm, Elena V. / Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging. в: Nanoscale. 2021 ; Том 13, № 23. стр. 10425-10435.

BibTeX

@article{25c8dd2497f5469c95ac9b9961273d79,
title = "Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging",
abstract = "Mesocrystals are nanostructured materials consisting of individual nanocrystals having a preferred crystallographic orientation. On mesoscopic length scales, the properties of mesocrystals are strongly affected by structural heterogeneity. Here, we report the detailed structural characterization of a faceted mesocrystal grain self-assembled from 60 nm sized gold nanocubes. Using coherent X-ray diffraction imaging, we determined the structure of the mesocrystal with the resolution sufficient to resolve each gold nanoparticle. The reconstructed electron density of the gold mesocrystal reveals its intrinsic structural heterogeneity, including local deviations of lattice parameters, and the presence of internal defects. The strain distribution shows that the average superlattice obtained by angular X-ray cross-correlation analysis and the real, {"}multidomain{"}structure of a mesocrystal are very close to each other, with a deviation less than 10%. These results will provide an important impact to understanding the fundamental principles of structuring and self-assembly including ensuing properties of mesocrystals.",
author = "Jerome Carnis and Felizitas Kirner and Dmitry Lapkin and Sebastian Sturm and Kim, {Young Yong} and Baburin, {Igor A.} and Ruslan Khubbutdinov and Alexandr Ignatenko and Ekaterina Iashina and Alexander Mistonov and Tristan Steegemans and Thomas Wieck and Thomas Gemming and Axel Lubk and Sergey Lazarev and Michael Sprung and Vartanyants, {Ivan A.} and Sturm, {Elena V.}",
note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry.",
year = "2021",
month = jun,
day = "21",
doi = "10.1039/d1nr01806j",
language = "English",
volume = "13",
pages = "10425--10435",
journal = "Nanoscale",
issn = "2040-3364",
publisher = "Royal Society of Chemistry",
number = "23",

}

RIS

TY - JOUR

T1 - Exploring the 3D structure and defects of a self-assembled gold mesocrystal by coherent X-ray diffraction imaging

AU - Carnis, Jerome

AU - Kirner, Felizitas

AU - Lapkin, Dmitry

AU - Sturm, Sebastian

AU - Kim, Young Yong

AU - Baburin, Igor A.

AU - Khubbutdinov, Ruslan

AU - Ignatenko, Alexandr

AU - Iashina, Ekaterina

AU - Mistonov, Alexander

AU - Steegemans, Tristan

AU - Wieck, Thomas

AU - Gemming, Thomas

AU - Lubk, Axel

AU - Lazarev, Sergey

AU - Sprung, Michael

AU - Vartanyants, Ivan A.

AU - Sturm, Elena V.

N1 - Publisher Copyright: © The Royal Society of Chemistry.

PY - 2021/6/21

Y1 - 2021/6/21

N2 - Mesocrystals are nanostructured materials consisting of individual nanocrystals having a preferred crystallographic orientation. On mesoscopic length scales, the properties of mesocrystals are strongly affected by structural heterogeneity. Here, we report the detailed structural characterization of a faceted mesocrystal grain self-assembled from 60 nm sized gold nanocubes. Using coherent X-ray diffraction imaging, we determined the structure of the mesocrystal with the resolution sufficient to resolve each gold nanoparticle. The reconstructed electron density of the gold mesocrystal reveals its intrinsic structural heterogeneity, including local deviations of lattice parameters, and the presence of internal defects. The strain distribution shows that the average superlattice obtained by angular X-ray cross-correlation analysis and the real, "multidomain"structure of a mesocrystal are very close to each other, with a deviation less than 10%. These results will provide an important impact to understanding the fundamental principles of structuring and self-assembly including ensuing properties of mesocrystals.

AB - Mesocrystals are nanostructured materials consisting of individual nanocrystals having a preferred crystallographic orientation. On mesoscopic length scales, the properties of mesocrystals are strongly affected by structural heterogeneity. Here, we report the detailed structural characterization of a faceted mesocrystal grain self-assembled from 60 nm sized gold nanocubes. Using coherent X-ray diffraction imaging, we determined the structure of the mesocrystal with the resolution sufficient to resolve each gold nanoparticle. The reconstructed electron density of the gold mesocrystal reveals its intrinsic structural heterogeneity, including local deviations of lattice parameters, and the presence of internal defects. The strain distribution shows that the average superlattice obtained by angular X-ray cross-correlation analysis and the real, "multidomain"structure of a mesocrystal are very close to each other, with a deviation less than 10%. These results will provide an important impact to understanding the fundamental principles of structuring and self-assembly including ensuing properties of mesocrystals.

UR - http://www.scopus.com/inward/record.url?scp=85108572538&partnerID=8YFLogxK

U2 - 10.1039/d1nr01806j

DO - 10.1039/d1nr01806j

M3 - Article

C2 - 34028473

AN - SCOPUS:85108572538

VL - 13

SP - 10425

EP - 10435

JO - Nanoscale

JF - Nanoscale

SN - 2040-3364

IS - 23

ER -

ID: 85654095