TY - JOUR

T1 - Collective excitations in spin-1/2 magnets through bond-operator formalism designed both for paramagnetic and ordered phases

AU - Сыромятников, Арсений Владиславович

N1 - Funding Information: We thank N. B. Christensen, D. Joshi, and O. P. Sushkov for exchange of data and useful discussions. This work is supported by Foundation for the advancement of theoretical physics and mathematics “BASIS.” APPENDIX:

PY - 2018/11/19

Y1 - 2018/11/19

N2 - We present a bond-operator theory (BOT) suitable for the description of both magnetically ordered phases and paramagnetic phases with singlet ground states in spin-1/2 magnets. This technique allows one to trace the evolution of quasiparticles across the transition between the phases. Some elementary excitations described in the theory by separate bosons appear in conventional approaches as bound states of well-known quasiparticles (magnons or triplons). The proposed BOT provides a regular expansion of physical quantities in powers of 1/n, where n is the maximum number of bosons that can occupy a unit cell (physical results correspond to n=1). Two variants of BOT are suggested: for two and for four spins in the unit cell (two-spin and four-spin BOTs, respectively). We consider spin-1/2 Heisenberg antiferromagnets (HAF) on a simple square lattice bilayer by the two-spin BOT. The ground-state energy E, the staggered magnetization M, and quasiparticle spectra found within the first order in 1/n are in good quantitative agreement with previous results both in paramagnetic and in ordered phases not very close to the quantum critical point between the phases. By doubling the unit cell in two directions, we discuss spin-1/2 HAF on a square lattice using the suggested four-spin BOT. We identify the magnon and the amplitude (Higgs) modes among fifteen spin-2, spin-1, and spin-0 quasiparticles arising in the theory. The magnon spectrum, E, and M found in the first order in 1/n are in good quantitative agreement with previous numerical and experimental results. We observe a special moderately damped spin-0 quasiparticle ("singlon" for short) whose energy is smaller than the energy of the Higgs mode in the most part of the Brillouin zone. By considering HAF with Ising-type anisotropy, we find that both Higgs and singlon modes stem from two-magnon bound states, which merge with two-magnon continuum not far from the isotropic limit. We demonstrate that singlons appear explicitly in "scalar" correlators one of which describes the Raman intensity in B1g symmetry. The latter is expressed in the leading order in 1/n via the singlon Green's function at zero momentum, which shows an asymmetric peak. The position of this peak given by the singlon energy coincides with the position of the so-called "two-magnon" peak observed experimentally in, e.g., layered cuprates.

AB - We present a bond-operator theory (BOT) suitable for the description of both magnetically ordered phases and paramagnetic phases with singlet ground states in spin-1/2 magnets. This technique allows one to trace the evolution of quasiparticles across the transition between the phases. Some elementary excitations described in the theory by separate bosons appear in conventional approaches as bound states of well-known quasiparticles (magnons or triplons). The proposed BOT provides a regular expansion of physical quantities in powers of 1/n, where n is the maximum number of bosons that can occupy a unit cell (physical results correspond to n=1). Two variants of BOT are suggested: for two and for four spins in the unit cell (two-spin and four-spin BOTs, respectively). We consider spin-1/2 Heisenberg antiferromagnets (HAF) on a simple square lattice bilayer by the two-spin BOT. The ground-state energy E, the staggered magnetization M, and quasiparticle spectra found within the first order in 1/n are in good quantitative agreement with previous results both in paramagnetic and in ordered phases not very close to the quantum critical point between the phases. By doubling the unit cell in two directions, we discuss spin-1/2 HAF on a square lattice using the suggested four-spin BOT. We identify the magnon and the amplitude (Higgs) modes among fifteen spin-2, spin-1, and spin-0 quasiparticles arising in the theory. The magnon spectrum, E, and M found in the first order in 1/n are in good quantitative agreement with previous numerical and experimental results. We observe a special moderately damped spin-0 quasiparticle ("singlon" for short) whose energy is smaller than the energy of the Higgs mode in the most part of the Brillouin zone. By considering HAF with Ising-type anisotropy, we find that both Higgs and singlon modes stem from two-magnon bound states, which merge with two-magnon continuum not far from the isotropic limit. We demonstrate that singlons appear explicitly in "scalar" correlators one of which describes the Raman intensity in B1g symmetry. The latter is expressed in the leading order in 1/n via the singlon Green's function at zero momentum, which shows an asymmetric peak. The position of this peak given by the singlon energy coincides with the position of the so-called "two-magnon" peak observed experimentally in, e.g., layered cuprates.

UR - http://www.scopus.com/inward/record.url?scp=85057186334&partnerID=8YFLogxK

U2 - 10.1103/PhysRevB.98.184421

DO - 10.1103/PhysRevB.98.184421

M3 - Article

VL - 98

JO - Physical Review B-Condensed Matter

JF - Physical Review B-Condensed Matter

SN - 1098-0121

IS - 18

M1 - 184421

ER -