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Asymmetric spin transitions of nonthermalized Mn2+ ions in (Zn,Mn)Se-based quantum wells. / Kudlacik, D.; Kavokin, K. V.; Lüders, C.; Barthelmi, K.; Schindler, J. J.; Moldenhauer, H.; Waldkirch, P.; Sapega, V. F.; Yakovlev, D. R.; Waag, A.; Bayer, M.; Debus, J.
в: Physical Review B, Том 101, № 15, 155432, 30.04.2020.Результаты исследований: Научные публикации в периодических изданиях › статья › Рецензирование
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TY - JOUR
T1 - Asymmetric spin transitions of nonthermalized Mn2+ ions in (Zn,Mn)Se-based quantum wells
AU - Kudlacik, D.
AU - Kavokin, K. V.
AU - Lüders, C.
AU - Barthelmi, K.
AU - Schindler, J. J.
AU - Moldenhauer, H.
AU - Waldkirch, P.
AU - Sapega, V. F.
AU - Yakovlev, D. R.
AU - Waag, A.
AU - Bayer, M.
AU - Debus, J.
N1 - Funding Information: We acknowledge financial support by the DFG and RFBR in the frame of the ICRC TRR 160 (Projects A6, B2, and B4). K.V.K. acknowledges a partial financial support by the St. Petersburg State University (Project No. 40.65.62.2017). Publisher Copyright: © 2020 American Physical Society. Copyright: Copyright 2020 Elsevier B.V., All rights reserved.
PY - 2020/4/30
Y1 - 2020/4/30
N2 - In Zn1-xMnxSe/(Zn,Be)Se quantum wells with x<0.035, nonthermalized Mn2+ ions demonstrate in spin-flip scattering spectra multiple Stokes and anti-Stokes transitions whose absolute energies deviate by up to 20% from each other. This asymmetry is tuned significantly by the optical power density, magnetic field direction, and Mn ion concentration. The nonequidistant Mn2+ spin transitions are modeled by the Zeeman splitting and quadrupolar crystal-field components taking values of up to 7 GHz. We suggest that nonequilibrium carriers dynamically polarize the Mn-ion spins so that they occupy levels with positive and negative spin projection numbers giving rise to asymmetric spin transitions.
AB - In Zn1-xMnxSe/(Zn,Be)Se quantum wells with x<0.035, nonthermalized Mn2+ ions demonstrate in spin-flip scattering spectra multiple Stokes and anti-Stokes transitions whose absolute energies deviate by up to 20% from each other. This asymmetry is tuned significantly by the optical power density, magnetic field direction, and Mn ion concentration. The nonequidistant Mn2+ spin transitions are modeled by the Zeeman splitting and quadrupolar crystal-field components taking values of up to 7 GHz. We suggest that nonequilibrium carriers dynamically polarize the Mn-ion spins so that they occupy levels with positive and negative spin projection numbers giving rise to asymmetric spin transitions.
KW - FLIP RAMAN-SCATTERING
KW - PARAMAGNETIC-RESONANCE
KW - EXCITATIONS
KW - DYNAMICS
KW - EXCITON
KW - STATES
UR - http://www.scopus.com/inward/record.url?scp=85084384261&partnerID=8YFLogxK
U2 - 10.1103/PhysRevB.101.155432
DO - 10.1103/PhysRevB.101.155432
M3 - Article
AN - SCOPUS:85084384261
VL - 101
JO - Physical Review B-Condensed Matter
JF - Physical Review B-Condensed Matter
SN - 1098-0121
IS - 15
M1 - 155432
ER -
ID: 70632862