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Two-photon Raman transition channels of NaCs predicted from ab initio calculations. / Wei, Jingbo; Li, Peng; Wu, Jizhou; Sovkov, Vladimir ; Liu, Wenliang; Li, Yuqing; Fu, Yongming; Xie, Feng; Ma, Jie.

In: Physical Review A - Atomic, Molecular, and Optical Physics, Vol. 105, No. 6, 063322, 22.06.2022.

Research output: Contribution to journalArticlepeer-review

Harvard

Wei, J, Li, P, Wu, J, Sovkov, V, Liu, W, Li, Y, Fu, Y, Xie, F & Ma, J 2022, 'Two-photon Raman transition channels of NaCs predicted from ab initio calculations', Physical Review A - Atomic, Molecular, and Optical Physics, vol. 105, no. 6, 063322. https://doi.org/10.1103/physreva.105.063322

APA

Wei, J., Li, P., Wu, J., Sovkov, V., Liu, W., Li, Y., Fu, Y., Xie, F., & Ma, J. (2022). Two-photon Raman transition channels of NaCs predicted from ab initio calculations. Physical Review A - Atomic, Molecular, and Optical Physics, 105(6), [063322]. https://doi.org/10.1103/physreva.105.063322

Vancouver

Wei J, Li P, Wu J, Sovkov V, Liu W, Li Y et al. Two-photon Raman transition channels of NaCs predicted from ab initio calculations. Physical Review A - Atomic, Molecular, and Optical Physics. 2022 Jun 22;105(6). 063322. https://doi.org/10.1103/physreva.105.063322

Author

Wei, Jingbo ; Li, Peng ; Wu, Jizhou ; Sovkov, Vladimir ; Liu, Wenliang ; Li, Yuqing ; Fu, Yongming ; Xie, Feng ; Ma, Jie. / Two-photon Raman transition channels of NaCs predicted from ab initio calculations. In: Physical Review A - Atomic, Molecular, and Optical Physics. 2022 ; Vol. 105, No. 6.

BibTeX

@article{feb5d2e5f9224021938e5e0039564af2,
title = "Two-photon Raman transition channels of NaCs predicted from ab initio calculations",
abstract = "Obtaining effective spontaneous radiative transition channels is a fundamental topic in the preparation of ultracold rovibrational ground states of molecules. Herein, the ranges of prospective transition channels in the NaCs dimer are predicted via exploring the complex energy level structure and transition properties. The potential energy curves of Λ-S states and ω states, spectroscopy constants, absolute energies of bound states, and transition information (Frank-Condon factors, lifetimes, transition dipole moments) have been researched. With this purpose, the results of our experiment on binding energies of the b3Π0+ rovibrational states are analyzed; the transition from the higher (photoassociated) 1Π state to the ground X1ς+ state is discussed. The wavelengths of the two lasers are predicted as 622.8-656.7 nm and 896.3-969.8 nm with the B1Π1 and c3ς1+ states, respectively, for the stimulated raman adiabatic passage method.",
author = "Jingbo Wei and Peng Li and Jizhou Wu and Vladimir Sovkov and Wenliang Liu and Yuqing Li and Yongming Fu and Feng Xie and Jie Ma",
note = "Publisher Copyright: {\textcopyright} 2022 American Physical Society.",
year = "2022",
month = jun,
day = "22",
doi = "10.1103/physreva.105.063322",
language = "English",
volume = "105",
journal = "Physical Review A - Atomic, Molecular, and Optical Physics",
issn = "1050-2947",
publisher = "American Physical Society",
number = "6",

}

RIS

TY - JOUR

T1 - Two-photon Raman transition channels of NaCs predicted from ab initio calculations

AU - Wei, Jingbo

AU - Li, Peng

AU - Wu, Jizhou

AU - Sovkov, Vladimir

AU - Liu, Wenliang

AU - Li, Yuqing

AU - Fu, Yongming

AU - Xie, Feng

AU - Ma, Jie

N1 - Publisher Copyright: © 2022 American Physical Society.

PY - 2022/6/22

Y1 - 2022/6/22

N2 - Obtaining effective spontaneous radiative transition channels is a fundamental topic in the preparation of ultracold rovibrational ground states of molecules. Herein, the ranges of prospective transition channels in the NaCs dimer are predicted via exploring the complex energy level structure and transition properties. The potential energy curves of Λ-S states and ω states, spectroscopy constants, absolute energies of bound states, and transition information (Frank-Condon factors, lifetimes, transition dipole moments) have been researched. With this purpose, the results of our experiment on binding energies of the b3Π0+ rovibrational states are analyzed; the transition from the higher (photoassociated) 1Π state to the ground X1ς+ state is discussed. The wavelengths of the two lasers are predicted as 622.8-656.7 nm and 896.3-969.8 nm with the B1Π1 and c3ς1+ states, respectively, for the stimulated raman adiabatic passage method.

AB - Obtaining effective spontaneous radiative transition channels is a fundamental topic in the preparation of ultracold rovibrational ground states of molecules. Herein, the ranges of prospective transition channels in the NaCs dimer are predicted via exploring the complex energy level structure and transition properties. The potential energy curves of Λ-S states and ω states, spectroscopy constants, absolute energies of bound states, and transition information (Frank-Condon factors, lifetimes, transition dipole moments) have been researched. With this purpose, the results of our experiment on binding energies of the b3Π0+ rovibrational states are analyzed; the transition from the higher (photoassociated) 1Π state to the ground X1ς+ state is discussed. The wavelengths of the two lasers are predicted as 622.8-656.7 nm and 896.3-969.8 nm with the B1Π1 and c3ς1+ states, respectively, for the stimulated raman adiabatic passage method.

UR - http://www.scopus.com/inward/record.url?scp=85133324665&partnerID=8YFLogxK

UR - https://www.mendeley.com/catalogue/73ce31c2-17ed-3e40-8808-075d26f1c45d/

U2 - 10.1103/physreva.105.063322

DO - 10.1103/physreva.105.063322

M3 - Article

VL - 105

JO - Physical Review A - Atomic, Molecular, and Optical Physics

JF - Physical Review A - Atomic, Molecular, and Optical Physics

SN - 1050-2947

IS - 6

M1 - 063322

ER -

ID: 96507977