• K. Kummer
  • C. Geibel
  • C. Krellner
  • G. Zwicknagl
  • C. Laubschat
  • N. B. Brookes
  • D. V. Vyalikh

The Kondo model predicts that both the valence at low temperatures and its temperature dependence scale with the characteristic energy T K of the Kondo interaction. Here, we study the evolution of the 4f occupancy with temperature in a series of Yb Kondo lattices using resonant X-ray emission spectroscopy. In agreement with simple theoretical models, we observe a scaling between the valence at low temperature and T K obtained from thermodynamic measurements. In contrast, the temperature scale T v at which the valence increases with temperature is almost the same in all investigated materials while the Kondo temperatures differ by almost four orders of magnitude. This observation is in remarkable contradiction to both naive expectation and precise theoretical predictions of the Kondo model, asking for further theoretical work in order to explain our findings. Our data exclude the presence of a quantum critical valence transition in YbRh2Si2.

Original languageEnglish
Article number2011
Number of pages7
JournalNature Communications
Volume9
Issue number1
DOIs
StatePublished - 22 May 2018

    Research areas

  • QUANTUM CRITICAL-POINT, 4F QUADRUPOLE-MOMENT, CRYSTAL-GROWTH, METAL YBRH2SI2, HEAVY, SUPERCONDUCTIVITY, DEPENDENCE, TRANSITION, YBIR2SI2, STATE

    Scopus subject areas

  • Physics and Astronomy(all)
  • Chemistry(all)
  • Biochemistry, Genetics and Molecular Biology(all)

ID: 36282841