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Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics. / Kouzov, A.; Radi, P.; Maksyutenko, P.; Kozlov, D.

In: Journal of Physics: Conference Series, Vol. 548, No. 1, 2014, p. 012016_1-5.

Research output: Contribution to journal › Article › peer-review

Harvard

Kouzov, A, Radi, P, Maksyutenko, P & Kozlov, D 2014, 'Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics', Journal of Physics: Conference Series, vol. 548, no. 1, pp. 012016_1-5. https://doi.org/doi:10.1088/1742-6596/548/1/012016

APA

Kouzov, A., Radi, P., Maksyutenko, P., & Kozlov, D. (2014). Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics. Journal of Physics: Conference Series, 548(1), 012016_1-5. https://doi.org/doi:10.1088/1742-6596/548/1/012016

Vancouver

Kouzov A, Radi P, Maksyutenko P, Kozlov D. Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics. Journal of Physics: Conference Series. 2014;548(1):012016_1-5. https://doi.org/doi:10.1088/1742-6596/548/1/012016

Author

Kouzov, A. ; Radi, P. ; Maksyutenko, P. ; Kozlov, D. / Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics. In: Journal of Physics: Conference Series. 2014 ; Vol. 548, No. 1. pp. 012016_1-5.

BibTeX

@article{bde504d6a147463bbfc5b23c27d8c81e,
title = "Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics",
abstract = "Frequency- and polarization-resolved degenerate resonant four-wave mixing is used for the first time to study the rotational anisotropy of the OH radicals produced by photolysis of H2O2 by a plane-polarized laser radiation at 266 nm. For that, a flexible polarization setup is designed to directly isolate the rotationally anisotropic signals in the A2Σ+X2Π(0; 0) OH vibronic band. The results are quantitatively interpreted by using the line-space approach and accounting for all possible correlations between the electric field ED of the photolysis laser, the recoil velocity v and the angular momentum J of nascent particles. In so doing, the resonance amplitudes are decoupled into products of the polarization factors, the Doppler-broadened profiles and the Einstein B-coefficients. The anisotropic signals have characteristic shapes of well resolved Doppler doublets providing a direct evidence of translational helicity of the nascent OH radicals, a hitherto exprementally inaccessible key characteristic of the photo",
keywords = "Four-wave mixing, photodissociation",
author = "A. Kouzov and P. Radi and P. Maksyutenko and D. Kozlov",
year = "2014",
doi = "doi:10.1088/1742-6596/548/1/012016",
language = "English",
volume = "548",
pages = "012016_1--5",
journal = "Journal of Physics: Conference Series",
issn = "1742-6588",
publisher = "IOP Publishing Ltd.",
number = "1",

}

RIS

TY - JOUR

T1 - Resonant four-wave mixing spectra: A fresh look at photodissociation dynamics

AU - Kouzov, A.

AU - Radi, P.

AU - Maksyutenko, P.

AU - Kozlov, D.

PY - 2014

Y1 - 2014

N2 - Frequency- and polarization-resolved degenerate resonant four-wave mixing is used for the first time to study the rotational anisotropy of the OH radicals produced by photolysis of H2O2 by a plane-polarized laser radiation at 266 nm. For that, a flexible polarization setup is designed to directly isolate the rotationally anisotropic signals in the A2Σ+X2Π(0; 0) OH vibronic band. The results are quantitatively interpreted by using the line-space approach and accounting for all possible correlations between the electric field ED of the photolysis laser, the recoil velocity v and the angular momentum J of nascent particles. In so doing, the resonance amplitudes are decoupled into products of the polarization factors, the Doppler-broadened profiles and the Einstein B-coefficients. The anisotropic signals have characteristic shapes of well resolved Doppler doublets providing a direct evidence of translational helicity of the nascent OH radicals, a hitherto exprementally inaccessible key characteristic of the photo

AB - Frequency- and polarization-resolved degenerate resonant four-wave mixing is used for the first time to study the rotational anisotropy of the OH radicals produced by photolysis of H2O2 by a plane-polarized laser radiation at 266 nm. For that, a flexible polarization setup is designed to directly isolate the rotationally anisotropic signals in the A2Σ+X2Π(0; 0) OH vibronic band. The results are quantitatively interpreted by using the line-space approach and accounting for all possible correlations between the electric field ED of the photolysis laser, the recoil velocity v and the angular momentum J of nascent particles. In so doing, the resonance amplitudes are decoupled into products of the polarization factors, the Doppler-broadened profiles and the Einstein B-coefficients. The anisotropic signals have characteristic shapes of well resolved Doppler doublets providing a direct evidence of translational helicity of the nascent OH radicals, a hitherto exprementally inaccessible key characteristic of the photo

KW - Four-wave mixing

KW - photodissociation

U2 - doi:10.1088/1742-6596/548/1/012016

DO - doi:10.1088/1742-6596/548/1/012016

M3 - Article

VL - 548

SP - 012016_1-5

JO - Journal of Physics: Conference Series

JF - Journal of Physics: Conference Series

SN - 1742-6588

IS - 1

ER -

ID: 5754363