The Møre and Vøring basins of the mid-Norwegian volcanic passive margin are characterized by thick accumulations of Cretaceous to Paleocene sedimentary strata. They were formed during a series of Late Mesozoic-Early Cenozoic extensional events and represent vast underexplored areas with a limited number of wells. Recently, a new generation of long-offset 2D seismic reflection lines and 3D seismic data, together with new well data, has permitted a significant improvement in the regional understanding of the Møre and Vøring basins. This has enabled much better imaging of the deep Cretaceous subbasins and sub-basalt structures. In light of this significant data improvement, we performed a regional tectonostratigraphic synthesis of the pre-breakup development of the Møre and Vøring basins. We have interpreted eight regional Cretaceous and Paleocene horizons and constructed a series of structural and thickness maps. The new interpretations allow us to examine the sequential evolution of the Cretaceous to Paleocene sedimentary infill and to discuss its relationship to the deep crustal structures and regional tectonic events. We conclude that the long and polyphased development of the Møre and Vøring basins is partly controlled by deep-seated structural highs. We show that active deposition in the Early Cretaceous was mainly focused in the Møre Basin, while the main Cenomanian and subsequent Late Cretaceous-Paleocene depocentres developed principally in the Vøring Basin and migrated sequentially west towards the present continent-ocean boundary. We argue that the outer Møre and Vøring basins are likely underlain by a relatively thick continental crust compared to the inner part of the regional sag basin. In this setting our observations do not support evidence for a large zone of exhumed upper mantle, which has previously been proposed to have formed before magmatism and breakup.