Research output: Contribution to journal › Article › peer-review
Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products. / Cui, Y.; Labidi, A.; Liang, X.; Huang, X.; Wang, J.; Li, X.; Dong, Q.; Zhang, X.; Othman, S.I.; Allam, A.A.; Bahnemann, D.W.; Wang, C.
In: ChemSusChem, Vol. 17, No. 18, 23.09.2024.Research output: Contribution to journal › Article › peer-review
}
TY - JOUR
T1 - Pivotal Impact Factors in Photocatalytic Reduction of CO2 to Value-Added C1 and C2 Products
AU - Cui, Y.
AU - Labidi, A.
AU - Liang, X.
AU - Huang, X.
AU - Wang, J.
AU - Li, X.
AU - Dong, Q.
AU - Zhang, X.
AU - Othman, S.I.
AU - Allam, A.A.
AU - Bahnemann, D.W.
AU - Wang, C.
N1 - Цитирования:3 Export Date: 19 October 2024 CODEN: CHEMI Адрес для корреспонденции: Bahnemann, D.W.; School of Environmental Science and Engineering, China; эл. почта: wangchuanyi@sust.edu.cn Адрес для корреспонденции: Wang, C.; School of Environmental Science and Engineering, China; эл. почта: cywang@ms.xjb.ac.cn Химические вещества/CAS: oxygen, 7782-44-7 Сведения о финансировании: National Natural Science Foundation of China, NSFC, 52161145409, 21976116 Сведения о финансировании: National Natural Science Foundation of China, NSFC Сведения о финансировании: 2023041004L, G2023041021L Текст о финансировании 1: . This work was supported by the National Natural Science Foundation of China ('52161145409, 21976116), SAFEA of China (\u201CBelt and Road\u201D Innovative Talent Exchange Foreign Expert Project # 2023041004L) (High\u2010end Foreign Expert Project # G2023041021L), and Alexander\u2010von\u2010Humboldt Foundation of Germany (Group\u2010Linkage Program). AOTP is thankful to the Phosagro/IUPAC/UNESCO research program in green chemistry. The authors acknowledge Princess Nourah bint Abdulrahman University Researchers Supporting Project number (PNURSP2024R5), Princess Nourah bint Abdulrahman University, Riyadh, Saudi Arabia
PY - 2024/9/23
Y1 - 2024/9/23
N2 - Over the past decades, CO2 greenhouse emission has been considerably increased, causing global warming and climate change. Indeed, converting CO2 into valuable chemicals and fuels is a desired option to resolve issues caused by its continuous emission into the atmosphere. Nevertheless, CO2 conversion has been hampered by the ultrahigh dissociation energy of C=O bonds, which makes it thermodynamically and kinetically challenging. From this prospect, photocatalytic approaches appear promising for CO2 reduction in terms of their efficiency compared to other traditional technologies. Thus, many efforts have been made in the designing of photocatalysts with asymmetric sites and oxygen vacancies, which can break the charge distribution balance of CO2 molecule, reduce hydrogenation energy barrier and accelerate CO2 conversion into chemicals and fuels. Here, we review the recent advances in CO2 hydrogenation to C1 and C2 products utilizing photocatalysis processes. We also pin down the key factors or parameters influencing the generation of C2 products during CO2 hydrogenation. In addition, the current status of CO2 reduction is summarized, projecting the future direction for CO2 conversion by photocatalysis processes. © 2024 Wiley-VCH GmbH.
AB - Over the past decades, CO2 greenhouse emission has been considerably increased, causing global warming and climate change. Indeed, converting CO2 into valuable chemicals and fuels is a desired option to resolve issues caused by its continuous emission into the atmosphere. Nevertheless, CO2 conversion has been hampered by the ultrahigh dissociation energy of C=O bonds, which makes it thermodynamically and kinetically challenging. From this prospect, photocatalytic approaches appear promising for CO2 reduction in terms of their efficiency compared to other traditional technologies. Thus, many efforts have been made in the designing of photocatalysts with asymmetric sites and oxygen vacancies, which can break the charge distribution balance of CO2 molecule, reduce hydrogenation energy barrier and accelerate CO2 conversion into chemicals and fuels. Here, we review the recent advances in CO2 hydrogenation to C1 and C2 products utilizing photocatalysis processes. We also pin down the key factors or parameters influencing the generation of C2 products during CO2 hydrogenation. In addition, the current status of CO2 reduction is summarized, projecting the future direction for CO2 conversion by photocatalysis processes. © 2024 Wiley-VCH GmbH.
KW - Asymmetric sites
KW - CO2 reduction
KW - Oxygen vacancies
KW - Photocatalysis
KW - Valuable chemicals
KW - Global warming
KW - Hydrogenation
KW - Asymmetric site
KW - CO 2 reduction
KW - Continuous emission
KW - Emissions into the atmosphere
KW - Global warming and climate changes
KW - Greenhouse emissions
KW - Impact factor
KW - Photocatalysis process
KW - Photocatalytic reduction
KW - Carbon dioxide
KW - fuel
KW - oxygen
KW - article
KW - atmosphere
KW - climate change
KW - dissociation
KW - greenhouse
KW - greenhouse effect
KW - hydrogenation
KW - kinetics
KW - photocatalysis
UR - https://www.mendeley.com/catalogue/0bed81aa-bfcb-38e8-bccc-df824b19550d/
U2 - 10.1002/cssc.202400551
DO - 10.1002/cssc.202400551
M3 - статья
VL - 17
JO - ChemSusChem
JF - ChemSusChem
SN - 1864-5631
IS - 18
ER -
ID: 126385795