Research output: Contribution to journal › Article › peer-review
Nonlinear Faraday effect and spin noise in rare-earth activated crystals. / Kamenskii, A. N.; Baibekov, E.I.; Kozlov, G. G. ; Malkin, B.Z.; Bayer, Manfred; Greilich, Alex; Zapasskii, V. S. .
In: Physical Review B-Condensed Matter, 11.2021.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Nonlinear Faraday effect and spin noise in rare-earth activated crystals
AU - Kamenskii, A. N.
AU - Baibekov, E.I.
AU - Kozlov, G. G.
AU - Malkin, B.Z.
AU - Bayer, Manfred
AU - Greilich, Alex
AU - Zapasskii, V. S.
PY - 2021/11
Y1 - 2021/11
N2 - The spin-noise spectroscopy (SNS) method implies high efficiency of conversion of the spin-system magnetization to the Faraday rotation angle. Generally, this efficiency cannot be estimated using the characteristics of the regular magneto-optical activity of a paramagnet. However, it may be drastically enhanced in systems with strong inhomogeneous broadening of the optical transitions. This enhancement leads to the giant spin-noise gain effect and previously allowed one to apply the SNS to rare-earth-activated crystals. We show that the nonlinear resonant Faraday effect can be used to measure the homogeneous width of the inhomogeneously broadened transition and, thus, to estimate the applicability of the SNS to this type of paramagnet. We present the theoretical description of the effect and perform measurements on intraconfigurational (4f-4f) transitions of the trivalent rare-earth ions of neodymium and ytterbium in fluorite-based crystals. The proposed experimental approach establishes new links between the effects of nonlinear optics and spin-noise characteristics of crystals with paramagnetic impurities and offers new ways of research in the physics of impurity crystals.
AB - The spin-noise spectroscopy (SNS) method implies high efficiency of conversion of the spin-system magnetization to the Faraday rotation angle. Generally, this efficiency cannot be estimated using the characteristics of the regular magneto-optical activity of a paramagnet. However, it may be drastically enhanced in systems with strong inhomogeneous broadening of the optical transitions. This enhancement leads to the giant spin-noise gain effect and previously allowed one to apply the SNS to rare-earth-activated crystals. We show that the nonlinear resonant Faraday effect can be used to measure the homogeneous width of the inhomogeneously broadened transition and, thus, to estimate the applicability of the SNS to this type of paramagnet. We present the theoretical description of the effect and perform measurements on intraconfigurational (4f-4f) transitions of the trivalent rare-earth ions of neodymium and ytterbium in fluorite-based crystals. The proposed experimental approach establishes new links between the effects of nonlinear optics and spin-noise characteristics of crystals with paramagnetic impurities and offers new ways of research in the physics of impurity crystals.
UR - https://journals.aps.org/prb/abstract/10.1103/PhysRevB.104.174430
M3 - Article
JO - Physical Review B-Condensed Matter
JF - Physical Review B-Condensed Matter
SN - 1098-0121
M1 - 174430
ER -
ID: 87967855