Research output: Contribution to journal › Article
Intra-center energy transfer dynamics in Cd1-xMnxTe semi magnetic semiconductors. / Vasilyev, Nikolay.
In: Journal of Luminescence, Vol. 132, No. 5, 2012, p. 1215-1219.Research output: Contribution to journal › Article
}
TY - JOUR
T1 - Intra-center energy transfer dynamics in Cd1-xMnxTe semi magnetic semiconductors
AU - Vasilyev, Nikolay
PY - 2012
Y1 - 2012
N2 - Intra-center luminescence of Cd1-xMnxTe semi magnetic semiconductors under low excitation density was investigated both experimentally and by Monte-Carlo simulation. Experimental time-resolved spectra of 2 eV-band under different photon energy for excitation were used. The approach revealed that Mn2+-Mn2+excitation energy transfers take place by means of resonant dipole-dipole interaction. Besides energy transfer dynamics is strongly influenced by hopping- assisted quenching. Having been intra-center excitation selective-, mixed- and non-selective types of excitation are proved to occur if photon energy for excitation is increased. This is originated from overlapping of 4T1- and 4T1-states. Under inter-band excitation it was established that Mn2+-ion excitation takes place with the aid of excitonic energy transfer, with excitation energy being centered at exciton energy. Under temperature rise the transfer rate vigorously enhances due to great increase of overlap integral of Mn2+- ions’ side-bands. The quench
AB - Intra-center luminescence of Cd1-xMnxTe semi magnetic semiconductors under low excitation density was investigated both experimentally and by Monte-Carlo simulation. Experimental time-resolved spectra of 2 eV-band under different photon energy for excitation were used. The approach revealed that Mn2+-Mn2+excitation energy transfers take place by means of resonant dipole-dipole interaction. Besides energy transfer dynamics is strongly influenced by hopping- assisted quenching. Having been intra-center excitation selective-, mixed- and non-selective types of excitation are proved to occur if photon energy for excitation is increased. This is originated from overlapping of 4T1- and 4T1-states. Under inter-band excitation it was established that Mn2+-ion excitation takes place with the aid of excitonic energy transfer, with excitation energy being centered at exciton energy. Under temperature rise the transfer rate vigorously enhances due to great increase of overlap integral of Mn2+- ions’ side-bands. The quench
KW - Cd1-xMnxTe
KW - Mn2+-luminescence
KW - energy transfer
KW - Monte-Carlo
KW - 4T1-state
U2 - 10.1016/j.jlumin.2011.12.047
DO - 10.1016/j.jlumin.2011.12.047
M3 - Article
VL - 132
SP - 1215
EP - 1219
JO - Journal of Luminescence
JF - Journal of Luminescence
SN - 0022-2313
IS - 5
ER -
ID: 5307237