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Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines. / Fu, Yunqi ; Zheng, Mang ; Li, Qi ; Zhang, Liping ; Wang, Shuai ; Kondratiev, V. V. ; Jiang, Baojiang.

In: RSC Advances, Vol. 47, No. 10, 18.07.2020, p. 28059-28065.

Research output: Contribution to journal › Article › peer-review

Harvard

Fu, Y, Zheng, M, Li, Q, Zhang, L, Wang, S, Kondratiev, VV & Jiang, B 2020, 'Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines', RSC Advances, vol. 47, no. 10, pp. 28059-28065.

APA

Fu, Y., Zheng, M., Li, Q., Zhang, L., Wang, S., Kondratiev, V. V., & Jiang, B. (2020). Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines. RSC Advances, 47(10), 28059-28065.

Vancouver

Fu Y, Zheng M, Li Q, Zhang L, Wang S, Kondratiev VV et al. Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines. RSC Advances. 2020 Jul 18;47(10):28059-28065.

Author

Fu, Yunqi ; Zheng, Mang ; Li, Qi ; Zhang, Liping ; Wang, Shuai ; Kondratiev, V. V. ; Jiang, Baojiang. / Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines. In: RSC Advances. 2020 ; Vol. 47, No. 10. pp. 28059-28065.

BibTeX

@article{caf18d465fe248fa8efe91394c5c4254,
title = "Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines",
abstract = "Benzylamine coupling is a very important reaction for the synthesis of imine but still faces many challenges.Herein, we present a highly effective strategy towards the coupling reaction by using environmentallyfriendly catalysts. These catalysts are composed of Cu/Cu2O/Cu3N heterostructures supported by C3N4tubes and the composites were synthesized by one-step hydrothermal treatment followed bycalcination. Cu2O, Cu3N, and C3N4 all are responsive to visible light and the heterojunction formed cangreatly enhance the charge separation. When used as photocatalysts for oxidative self-coupling ofbenzylamine at a low temperature of 323 K in air, Cu/Cu2O/Cu3N/C3N4 was able to give conversion andselectivity values of up to 99% and 98%, respectively. The high efficiency of the catalysts is attributable totheir ability to generate large quantities of free radicals (such as $OH and $O2) under visible-light irradiation",
keywords = "photocatalytic oxidation , heterostructures",
author = "Yunqi Fu and Mang Zheng and Qi Li and Liping Zhang and Shuai Wang and Kondratiev, {V. V.} and Baojiang Jiang",
year = "2020",
month = jul,
day = "18",
language = "English",
volume = "47",
pages = "28059--28065",
journal = "RSC Advances",
issn = "2046-2069",
publisher = "Royal Society of Chemistry",
number = "10",

}

RIS

TY - JOUR

T1 - Interfacial engineering by creating Cu-based ternary heterostructures on C3N4 tubes towards enhanced photocatalytic oxidative coupling of benzylamines

AU - Fu, Yunqi

AU - Zheng, Mang

AU - Li, Qi

AU - Zhang, Liping

AU - Wang, Shuai

AU - Kondratiev, V. V.

AU - Jiang, Baojiang

PY - 2020/7/18

Y1 - 2020/7/18

N2 - Benzylamine coupling is a very important reaction for the synthesis of imine but still faces many challenges.Herein, we present a highly effective strategy towards the coupling reaction by using environmentallyfriendly catalysts. These catalysts are composed of Cu/Cu2O/Cu3N heterostructures supported by C3N4tubes and the composites were synthesized by one-step hydrothermal treatment followed bycalcination. Cu2O, Cu3N, and C3N4 all are responsive to visible light and the heterojunction formed cangreatly enhance the charge separation. When used as photocatalysts for oxidative self-coupling ofbenzylamine at a low temperature of 323 K in air, Cu/Cu2O/Cu3N/C3N4 was able to give conversion andselectivity values of up to 99% and 98%, respectively. The high efficiency of the catalysts is attributable totheir ability to generate large quantities of free radicals (such as $OH and $O2) under visible-light irradiation

AB - Benzylamine coupling is a very important reaction for the synthesis of imine but still faces many challenges.Herein, we present a highly effective strategy towards the coupling reaction by using environmentallyfriendly catalysts. These catalysts are composed of Cu/Cu2O/Cu3N heterostructures supported by C3N4tubes and the composites were synthesized by one-step hydrothermal treatment followed bycalcination. Cu2O, Cu3N, and C3N4 all are responsive to visible light and the heterojunction formed cangreatly enhance the charge separation. When used as photocatalysts for oxidative self-coupling ofbenzylamine at a low temperature of 323 K in air, Cu/Cu2O/Cu3N/C3N4 was able to give conversion andselectivity values of up to 99% and 98%, respectively. The high efficiency of the catalysts is attributable totheir ability to generate large quantities of free radicals (such as $OH and $O2) under visible-light irradiation

KW - photocatalytic oxidation , heterostructures

UR - https://pubs.rsc.org/en/Content/ArticleLanding/2020/RA/D0RA03164J#!divAbstract

M3 - Article

VL - 47

SP - 28059

EP - 28065

JO - RSC Advances

JF - RSC Advances

SN - 2046-2069

IS - 10

ER -

ID: 62104538