We present a new approach for the preparation of electrocatalytically active carbonaceous coatings embedding bimetallic nanoparticles (NPs) - AgPt@C structures, on surfaces with 2D and 3D geometry such as glass covered with indium tin oxide (ITO) film and anodic aluminum oxide substrates, respectively. We provide extensive characterization of the deposited structures and demonstrate their performance towards the electrocatalytic glucose oxidation, one half-reaction of biofuel cells. We observe that a preliminary surface treatment of the porous alumina substrate is essential for a homogeneous laser-induced deposition of AgPt@C nanoparticles across the whole pore depth.