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Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics. / Burt, Michael; Boll, Rebecca; Lee, Jason W. L.; Amini, Kasra; Kockert, Hansjochen; Vallance, Claire; Gentleman, Alexander S.; Mackenzie, Stuart R.; Bari, Sadia; Bomme, Cedric; Duesterer, Stefan; Erk, Benjamin; Manschwetus, Bastian; Mueller, Erland; Rompotis, Dimitrios; Savelyev, Evgeny; Schirmel, Nora; Techert, Simone; Treusch, Rolf; Kuepper, Jochen; Trippel, Sebastian; Wiese, Joss; Stapelfeldt, Henrik; de Miranda, Barbara Cunha; Guillemin, Renaud; Ismail, Iyas; Journel, Loic; Marchenko, Tatiana; Palaudoux, Jerome; Penent, Francis; Piancastelli, Maria Novella; Simon, Marc; Travnikova, Oksana; Brausse, Felix; Goldsztejn, Gildas; Rouzee, Arnaud; Geleoc, Marie; Geneaux, Romain; Ruchon, Thierry; Underwood, Jonathan; Holland, David M. P.; Mereshchenko, Andrey S.; Olshin, Pavel K.; Johnsson, Per; Maclot, Sylvain; Lahl, Jan; Rudenko, Artem; Ziaee, Farzaneh; Brouard, Mark; Rolles, Daniel.
In:
Physical Review A, Vol. 96, No. 4, 043415, 17.10.2017.
Research output: Contribution to journal › Article › peer-review
Harvard
Burt, M, Boll, R, Lee, JWL, Amini, K, Kockert, H, Vallance, C, Gentleman, AS, Mackenzie, SR, Bari, S, Bomme, C, Duesterer, S, Erk, B, Manschwetus, B, Mueller, E, Rompotis, D, Savelyev, E, Schirmel, N, Techert, S, Treusch, R, Kuepper, J, Trippel, S, Wiese, J, Stapelfeldt, H, de Miranda, BC, Guillemin, R, Ismail, I, Journel, L, Marchenko, T, Palaudoux, J, Penent, F, Piancastelli, MN, Simon, M, Travnikova, O, Brausse, F, Goldsztejn, G, Rouzee, A, Geleoc, M, Geneaux, R, Ruchon, T, Underwood, J, Holland, DMP
, Mereshchenko, AS, Olshin, PK, Johnsson, P, Maclot, S, Lahl, J, Rudenko, A, Ziaee, F, Brouard, M & Rolles, D 2017, '
Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics',
Physical Review A, vol. 96, no. 4, 043415.
https://doi.org/10.1103/PhysRevA.96.043415APA
Burt, M., Boll, R., Lee, J. W. L., Amini, K., Kockert, H., Vallance, C., Gentleman, A. S., Mackenzie, S. R., Bari, S., Bomme, C., Duesterer, S., Erk, B., Manschwetus, B., Mueller, E., Rompotis, D., Savelyev, E., Schirmel, N., Techert, S., Treusch, R., ... Rolles, D. (2017).
Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics.
Physical Review A,
96(4), [043415].
https://doi.org/10.1103/PhysRevA.96.043415Vancouver
Author
Burt, Michael ; Boll, Rebecca ; Lee, Jason W. L. ; Amini, Kasra ; Kockert, Hansjochen ; Vallance, Claire ; Gentleman, Alexander S. ; Mackenzie, Stuart R. ; Bari, Sadia ; Bomme, Cedric ; Duesterer, Stefan ; Erk, Benjamin ; Manschwetus, Bastian ; Mueller, Erland ; Rompotis, Dimitrios ; Savelyev, Evgeny ; Schirmel, Nora ; Techert, Simone ; Treusch, Rolf ; Kuepper, Jochen ; Trippel, Sebastian ; Wiese, Joss ; Stapelfeldt, Henrik ; de Miranda, Barbara Cunha ; Guillemin, Renaud ; Ismail, Iyas ; Journel, Loic ; Marchenko, Tatiana ; Palaudoux, Jerome ; Penent, Francis ; Piancastelli, Maria Novella ; Simon, Marc ; Travnikova, Oksana ; Brausse, Felix ; Goldsztejn, Gildas ; Rouzee, Arnaud ; Geleoc, Marie ; Geneaux, Romain ; Ruchon, Thierry ; Underwood, Jonathan ; Holland, David M. P.
; Mereshchenko, Andrey S. ; Olshin, Pavel K. ; Johnsson, Per ; Maclot, Sylvain ; Lahl, Jan ; Rudenko, Artem ; Ziaee, Farzaneh ; Brouard, Mark ; Rolles, Daniel. /
Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics. In:
Physical Review A. 2017 ; Vol. 96, No. 4.
BibTeX
@article{7e0aa5d5f3cf4d8081fd9bf8ba8701da,
title = "Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics",
abstract = "The dynamics following laser-induced molecular photodissociation of gas-phase CH2BrI at 271.6 nm were investigated by time-resolved Coulomb-explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH2BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of C(H)2Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb-explosion imaging as a real-time probe of chemical dynamics.",
keywords = "LASER-FIELD, 193 NM, CHLOROIODOMETHANE, PHOTOELECTRON, ULTRAVIOLET, IONIZATION, MOLECULES, PULSES, CH2ICL, CH3I",
author = "Michael Burt and Rebecca Boll and Lee, {Jason W. L.} and Kasra Amini and Hansjochen Kockert and Claire Vallance and Gentleman, {Alexander S.} and Mackenzie, {Stuart R.} and Sadia Bari and Cedric Bomme and Stefan Duesterer and Benjamin Erk and Bastian Manschwetus and Erland Mueller and Dimitrios Rompotis and Evgeny Savelyev and Nora Schirmel and Simone Techert and Rolf Treusch and Jochen Kuepper and Sebastian Trippel and Joss Wiese and Henrik Stapelfeldt and {de Miranda}, {Barbara Cunha} and Renaud Guillemin and Iyas Ismail and Loic Journel and Tatiana Marchenko and Jerome Palaudoux and Francis Penent and Piancastelli, {Maria Novella} and Marc Simon and Oksana Travnikova and Felix Brausse and Gildas Goldsztejn and Arnaud Rouzee and Marie Geleoc and Romain Geneaux and Thierry Ruchon and Jonathan Underwood and Holland, {David M. P.} and Mereshchenko, {Andrey S.} and Olshin, {Pavel K.} and Per Johnsson and Sylvain Maclot and Jan Lahl and Artem Rudenko and Farzaneh Ziaee and Mark Brouard and Daniel Rolles",
year = "2017",
month = oct,
day = "17",
doi = "10.1103/PhysRevA.96.043415",
language = "Английский",
volume = "96",
journal = "Physical Review A - Atomic, Molecular, and Optical Physics",
issn = "1050-2947",
publisher = "American Physical Society",
number = "4",
}
RIS
TY - JOUR
T1 - Coulomb-explosion imaging of concurrent CH2BrI photodissociation dynamics
AU - Burt, Michael
AU - Boll, Rebecca
AU - Lee, Jason W. L.
AU - Amini, Kasra
AU - Kockert, Hansjochen
AU - Vallance, Claire
AU - Gentleman, Alexander S.
AU - Mackenzie, Stuart R.
AU - Bari, Sadia
AU - Bomme, Cedric
AU - Duesterer, Stefan
AU - Erk, Benjamin
AU - Manschwetus, Bastian
AU - Mueller, Erland
AU - Rompotis, Dimitrios
AU - Savelyev, Evgeny
AU - Schirmel, Nora
AU - Techert, Simone
AU - Treusch, Rolf
AU - Kuepper, Jochen
AU - Trippel, Sebastian
AU - Wiese, Joss
AU - Stapelfeldt, Henrik
AU - de Miranda, Barbara Cunha
AU - Guillemin, Renaud
AU - Ismail, Iyas
AU - Journel, Loic
AU - Marchenko, Tatiana
AU - Palaudoux, Jerome
AU - Penent, Francis
AU - Piancastelli, Maria Novella
AU - Simon, Marc
AU - Travnikova, Oksana
AU - Brausse, Felix
AU - Goldsztejn, Gildas
AU - Rouzee, Arnaud
AU - Geleoc, Marie
AU - Geneaux, Romain
AU - Ruchon, Thierry
AU - Underwood, Jonathan
AU - Holland, David M. P.
AU - Mereshchenko, Andrey S.
AU - Olshin, Pavel K.
AU - Johnsson, Per
AU - Maclot, Sylvain
AU - Lahl, Jan
AU - Rudenko, Artem
AU - Ziaee, Farzaneh
AU - Brouard, Mark
AU - Rolles, Daniel
PY - 2017/10/17
Y1 - 2017/10/17
N2 - The dynamics following laser-induced molecular photodissociation of gas-phase CH2BrI at 271.6 nm were investigated by time-resolved Coulomb-explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH2BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of C(H)2Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb-explosion imaging as a real-time probe of chemical dynamics.
AB - The dynamics following laser-induced molecular photodissociation of gas-phase CH2BrI at 271.6 nm were investigated by time-resolved Coulomb-explosion imaging using intense near-IR femtosecond laser pulses. The observed delay-dependent photofragment momenta reveal that CH2BrI undergoes C-I cleavage, depositing 65.6% of the available energy into internal product states, and that absorption of a second UV photon breaks the C-Br bond of C(H)2Br. Simulations confirm that this mechanism is consistent with previous data recorded at 248 nm, demonstrating the sensitivity of Coulomb-explosion imaging as a real-time probe of chemical dynamics.
KW - LASER-FIELD
KW - 193 NM
KW - CHLOROIODOMETHANE
KW - PHOTOELECTRON
KW - ULTRAVIOLET
KW - IONIZATION
KW - MOLECULES
KW - PULSES
KW - CH2ICL
KW - CH3I
U2 - 10.1103/PhysRevA.96.043415
DO - 10.1103/PhysRevA.96.043415
M3 - статья
VL - 96
JO - Physical Review A - Atomic, Molecular, and Optical Physics
JF - Physical Review A - Atomic, Molecular, and Optical Physics
SN - 1050-2947
IS - 4
M1 - 043415
ER -
