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Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics. / Allum, Felix; Burt, Michael; Amini, Kasra; Boll, Rebecca; Köckert, Hansjochen; Olshin, Pavel K.; Bari, Sadia; Bomme, Cédric; Brauße, Felix; Cunha de Miranda, Barbara; Düsterer, Stefan; Erk, Benjamin; Géléoc, Marie; Geneaux, Romain; Gentleman, Alexander S.; Goldsztejn, Gildas; Guillemin, Renaud; Holland, David M.P.; Ismail, Iyas; Johnsson, Per; Journel, Loïc; Küpper, Jochen; Lahl, Jan; Lee, Jason W.L.; Maclot, Sylvain; Mackenzie, Stuart R.; Manschwetus, Bastian; Mereshchenko, Andrey S.; Mason, Robert; Palaudoux, Jérôme; Piancastelli, Maria Novella; Penent, Francis; Rompotis, Dimitrios; Rouzée, Arnaud; Ruchon, Thierry; Rudenko, Artem; Savelyev, Evgeny; Simon, Marc; Schirmel, Nora; Stapelfeldt, Henrik; Techert, Simone; Travnikova, Oksana; Trippel, Sebastian; Underwood, Jonathan G.; Vallance, Claire; Wiese, Joss; Ziaee, Farzaneh; Brouard, Mark; Marchenko, Tatiana; Rolles, Daniel.

In: The Journal of Chemical Physics, Vol. 149, No. 20, 204313, 28.11.2018.

Research output: Contribution to journal › Article › peer-review

Harvard

Allum, F, Burt, M, Amini, K, Boll, R, Köckert, H, Olshin, PK, Bari, S, Bomme, C, Brauße, F, Cunha de Miranda, B, Düsterer, S, Erk, B, Géléoc, M, Geneaux, R, Gentleman, AS, Goldsztejn, G, Guillemin, R, Holland, DMP, Ismail, I, Johnsson, P, Journel, L, Küpper, J, Lahl, J, Lee, JWL, Maclot, S, Mackenzie, SR, Manschwetus, B, Mereshchenko, AS, Mason, R, Palaudoux, J, Piancastelli, MN, Penent, F, Rompotis, D, Rouzée, A, Ruchon, T, Rudenko, A, Savelyev, E, Simon, M, Schirmel, N, Stapelfeldt, H, Techert, S, Travnikova, O, Trippel, S, Underwood, JG, Vallance, C, Wiese, J, Ziaee, F, Brouard, M, Marchenko, T & Rolles, D 2018, 'Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics', The Journal of Chemical Physics, vol. 149, no. 20, 204313. https://doi.org/10.1063/1.5041381

APA

Allum, F., Burt, M., Amini, K., Boll, R., Köckert, H., Olshin, P. K., Bari, S., Bomme, C., Brauße, F., Cunha de Miranda, B., Düsterer, S., Erk, B., Géléoc, M., Geneaux, R., Gentleman, A. S., Goldsztejn, G., Guillemin, R., Holland, D. M. P., Ismail, I., ... Rolles, D. (2018). Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics. The Journal of Chemical Physics, 149(20), [204313]. https://doi.org/10.1063/1.5041381

Vancouver

Allum F, Burt M, Amini K, Boll R, Köckert H, Olshin PK et al. Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics. The Journal of Chemical Physics. 2018 Nov 28;149(20). 204313. https://doi.org/10.1063/1.5041381

Author

Allum, Felix ; Burt, Michael ; Amini, Kasra ; Boll, Rebecca ; Köckert, Hansjochen ; Olshin, Pavel K. ; Bari, Sadia ; Bomme, Cédric ; Brauße, Felix ; Cunha de Miranda, Barbara ; Düsterer, Stefan ; Erk, Benjamin ; Géléoc, Marie ; Geneaux, Romain ; Gentleman, Alexander S. ; Goldsztejn, Gildas ; Guillemin, Renaud ; Holland, David M.P. ; Ismail, Iyas ; Johnsson, Per ; Journel, Loïc ; Küpper, Jochen ; Lahl, Jan ; Lee, Jason W.L. ; Maclot, Sylvain ; Mackenzie, Stuart R. ; Manschwetus, Bastian ; Mereshchenko, Andrey S. ; Mason, Robert ; Palaudoux, Jérôme ; Piancastelli, Maria Novella ; Penent, Francis ; Rompotis, Dimitrios ; Rouzée, Arnaud ; Ruchon, Thierry ; Rudenko, Artem ; Savelyev, Evgeny ; Simon, Marc ; Schirmel, Nora ; Stapelfeldt, Henrik ; Techert, Simone ; Travnikova, Oksana ; Trippel, Sebastian ; Underwood, Jonathan G. ; Vallance, Claire ; Wiese, Joss ; Ziaee, Farzaneh ; Brouard, Mark ; Marchenko, Tatiana ; Rolles, Daniel. / Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics. In: The Journal of Chemical Physics. 2018 ; Vol. 149, No. 20.

BibTeX

@article{92560b0844024138bf7f508ef34c1b15,
title = "Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics",
abstract = "The photodissociation dynamics of CH3I and CH2ClI at 272 nm were investigated by time-resolved Coulomb explosion imaging, with an intense non-resonant 815 nm probe pulse. Fragment ion momenta over a wide m/z range were recorded simultaneously by coupling a velocity map imaging spectrometer with a pixel imaging mass spectrometry camera. For both molecules, delay-dependent pump-probe features were assigned to ultraviolet-induced carbon-iodine bond cleavage followed by Coulomb explosion. Multi-mass imaging also allowed the sequential cleavage of both carbon-halogen bonds in CH2ClI to be investigated. Furthermore, delay-dependent relative fragment momenta of a pair of ions were directly determined using recoil-frame covariance analysis. These results are complementary to conventional velocity map imaging experiments and demonstrate the application of time-resolved Coulomb explosion imaging to photoinduced real-time molecular motion.",
keywords = "METHYL-IODIDE, VELOCITY, BAND, CHLOROIODOMETHANE, SPECTROSCOPY, ABSORPTION, CIS, PHOTOFRAGMENTATION, PHOTOELECTRON, EXCITATION",
author = "Felix Allum and Michael Burt and Kasra Amini and Rebecca Boll and Hansjochen K{\"o}ckert and Olshin, {Pavel K.} and Sadia Bari and C{\'e}dric Bomme and Felix Brau{\ss}e and {Cunha de Miranda}, Barbara and Stefan D{\"u}sterer and Benjamin Erk and Marie G{\'e}l{\'e}oc and Romain Geneaux and Gentleman, {Alexander S.} and Gildas Goldsztejn and Renaud Guillemin and Holland, {David M.P.} and Iyas Ismail and Per Johnsson and Lo{\"i}c Journel and Jochen K{\"u}pper and Jan Lahl and Lee, {Jason W.L.} and Sylvain Maclot and Mackenzie, {Stuart R.} and Bastian Manschwetus and Mereshchenko, {Andrey S.} and Robert Mason and J{\'e}r{\^o}me Palaudoux and Piancastelli, {Maria Novella} and Francis Penent and Dimitrios Rompotis and Arnaud Rouz{\'e}e and Thierry Ruchon and Artem Rudenko and Evgeny Savelyev and Marc Simon and Nora Schirmel and Henrik Stapelfeldt and Simone Techert and Oksana Travnikova and Sebastian Trippel and Underwood, {Jonathan G.} and Claire Vallance and Joss Wiese and Farzaneh Ziaee and Mark Brouard and Tatiana Marchenko and Daniel Rolles",
note = "doi: 10.1063/1.5041381",
year = "2018",
month = nov,
day = "28",
doi = "10.1063/1.5041381",
language = "English",
volume = "149",
journal = "Journal of Chemical Physics",
issn = "0021-9606",
publisher = "American Institute of Physics",
number = "20",

}

RIS

TY - JOUR

T1 - Coulomb explosion imaging of CH3I and CH2ClI photodissociation dynamics

AU - Allum, Felix

AU - Burt, Michael

AU - Amini, Kasra

AU - Boll, Rebecca

AU - Köckert, Hansjochen

AU - Olshin, Pavel K.

AU - Bari, Sadia

AU - Bomme, Cédric

AU - Brauße, Felix

AU - Cunha de Miranda, Barbara

AU - Düsterer, Stefan

AU - Erk, Benjamin

AU - Géléoc, Marie

AU - Geneaux, Romain

AU - Gentleman, Alexander S.

AU - Goldsztejn, Gildas

AU - Guillemin, Renaud

AU - Holland, David M.P.

AU - Ismail, Iyas

AU - Johnsson, Per

AU - Journel, Loïc

AU - Küpper, Jochen

AU - Lahl, Jan

AU - Lee, Jason W.L.

AU - Maclot, Sylvain

AU - Mackenzie, Stuart R.

AU - Manschwetus, Bastian

AU - Mereshchenko, Andrey S.

AU - Mason, Robert

AU - Palaudoux, Jérôme

AU - Piancastelli, Maria Novella

AU - Penent, Francis

AU - Rompotis, Dimitrios

AU - Rouzée, Arnaud

AU - Ruchon, Thierry

AU - Rudenko, Artem

AU - Savelyev, Evgeny

AU - Simon, Marc

AU - Schirmel, Nora

AU - Stapelfeldt, Henrik

AU - Techert, Simone

AU - Travnikova, Oksana

AU - Trippel, Sebastian

AU - Underwood, Jonathan G.

AU - Vallance, Claire

AU - Wiese, Joss

AU - Ziaee, Farzaneh

AU - Brouard, Mark

AU - Marchenko, Tatiana

AU - Rolles, Daniel

N1 - doi: 10.1063/1.5041381

PY - 2018/11/28

Y1 - 2018/11/28

N2 - The photodissociation dynamics of CH3I and CH2ClI at 272 nm were investigated by time-resolved Coulomb explosion imaging, with an intense non-resonant 815 nm probe pulse. Fragment ion momenta over a wide m/z range were recorded simultaneously by coupling a velocity map imaging spectrometer with a pixel imaging mass spectrometry camera. For both molecules, delay-dependent pump-probe features were assigned to ultraviolet-induced carbon-iodine bond cleavage followed by Coulomb explosion. Multi-mass imaging also allowed the sequential cleavage of both carbon-halogen bonds in CH2ClI to be investigated. Furthermore, delay-dependent relative fragment momenta of a pair of ions were directly determined using recoil-frame covariance analysis. These results are complementary to conventional velocity map imaging experiments and demonstrate the application of time-resolved Coulomb explosion imaging to photoinduced real-time molecular motion.

AB - The photodissociation dynamics of CH3I and CH2ClI at 272 nm were investigated by time-resolved Coulomb explosion imaging, with an intense non-resonant 815 nm probe pulse. Fragment ion momenta over a wide m/z range were recorded simultaneously by coupling a velocity map imaging spectrometer with a pixel imaging mass spectrometry camera. For both molecules, delay-dependent pump-probe features were assigned to ultraviolet-induced carbon-iodine bond cleavage followed by Coulomb explosion. Multi-mass imaging also allowed the sequential cleavage of both carbon-halogen bonds in CH2ClI to be investigated. Furthermore, delay-dependent relative fragment momenta of a pair of ions were directly determined using recoil-frame covariance analysis. These results are complementary to conventional velocity map imaging experiments and demonstrate the application of time-resolved Coulomb explosion imaging to photoinduced real-time molecular motion.

KW - METHYL-IODIDE

KW - VELOCITY

KW - BAND

KW - CHLOROIODOMETHANE

KW - SPECTROSCOPY

KW - ABSORPTION

KW - CIS

KW - PHOTOFRAGMENTATION

KW - PHOTOELECTRON

KW - EXCITATION

UR - http://www.scopus.com/inward/record.url?scp=85057771736&partnerID=8YFLogxK

U2 - 10.1063/1.5041381

DO - 10.1063/1.5041381

M3 - Article

C2 - 30501230

VL - 149

JO - Journal of Chemical Physics

JF - Journal of Chemical Physics

SN - 0021-9606

IS - 20

M1 - 204313

ER -

ID: 36476492