Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review
Controlling the emission time of photon echoes by optical freezing of exciton dephasing and rephasing in quantum-dot ensembles. / Reichelt, Matthias; Rose, Hendrik; Kosarev, Alexander N.; Poltavtsev, Sergey V.; Bayer, Manfred; Akimov, Ilya A.; Schneider, Christian; Kamp, Martin; Höfling, Sven; Meier, Torsten.
Proceedings of SPIE - The International Society for Optical Engineering. ed. / Markus Betz; Abdulhakem Y. Elezzabi. Vol. 11684 SPIE, 2021. 116840X.Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review
}
TY - GEN
T1 - Controlling the emission time of photon echoes by optical freezing of exciton dephasing and rephasing in quantum-dot ensembles
AU - Reichelt, Matthias
AU - Rose, Hendrik
AU - Kosarev, Alexander N.
AU - Poltavtsev, Sergey V.
AU - Bayer, Manfred
AU - Akimov, Ilya A.
AU - Schneider, Christian
AU - Kamp, Martin
AU - Höfling, Sven
AU - Meier, Torsten
N1 - Funding Information: We acknowledge financial support from the Deutsche Forschungsgemeinschaft (DFG) through the Collaborative Research Center TRR 142 (Project number 231447078, project A02). S.V.P. thanks the Russian Foundation for Basic Research (Project number 19-52-12046) and the Saint Petersburg State University (Grant number 51125686). The Würzburg group acknowledges financial support by the state of Bavaria. Publisher Copyright: © 2021 SPIE.
PY - 2021/3/5
Y1 - 2021/3/5
N2 - Following the ultrafast optical excitation of an inhomogeneously broadened ensemble, the macroscopic optical polarization decays rapidly due to dephasing. This destructive interference is, however, reversible in photon echo experiments. Here, we propose a concept in which a control pulse slows down either the dephasing or the rephasing of the exciton ensemble during its presence. We analyze and visualize this optical freezing process by showing and discussing results for different single and multiple sequences of control pulses using a simple model of inhomogeneously broadened two-level systems. This idea has been realized in experiments performed on self-assembled (In,Ga)As quantum dots where it was possible to retard or advance the photon echo emission time by several picoseconds. The measurements are in very good agreement with numerical simulations for a more realistic model which, in particular, takes the spatial shape of the laser pulses into account.
AB - Following the ultrafast optical excitation of an inhomogeneously broadened ensemble, the macroscopic optical polarization decays rapidly due to dephasing. This destructive interference is, however, reversible in photon echo experiments. Here, we propose a concept in which a control pulse slows down either the dephasing or the rephasing of the exciton ensemble during its presence. We analyze and visualize this optical freezing process by showing and discussing results for different single and multiple sequences of control pulses using a simple model of inhomogeneously broadened two-level systems. This idea has been realized in experiments performed on self-assembled (In,Ga)As quantum dots where it was possible to retard or advance the photon echo emission time by several picoseconds. The measurements are in very good agreement with numerical simulations for a more realistic model which, in particular, takes the spatial shape of the laser pulses into account.
KW - four-wave mixing
KW - inhomogeneous broadening
KW - Nonlinear optics
KW - optical Bloch equations
KW - optical control
KW - photon echo
KW - quantum dots
UR - http://www.scopus.com/inward/record.url?scp=85105918115&partnerID=8YFLogxK
UR - https://www.mendeley.com/catalogue/17eae6ec-26ee-3f36-b445-a18fd89c816c/
U2 - 10.1117/12.2576887
DO - 10.1117/12.2576887
M3 - Conference contribution
AN - SCOPUS:85105918115
VL - 11684
BT - Proceedings of SPIE - The International Society for Optical Engineering
A2 - Betz, Markus
A2 - Elezzabi, Abdulhakem Y.
PB - SPIE
T2 - Ultrafast Phenomena and Nanophotonics XXV 2021
Y2 - 6 March 2021 through 11 March 2021
ER -
ID: 86056304