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Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals. / Belykh, Vasilii V.; Yakovlev, Dmitri R.; Glazov, Mikhail M.; Grigoryev, Philipp S.; Hussain, Mujtaba; Rautert, Janina; Dirin, Dmitry N.; Kovalenko, Maksym V.; Bayer, Manfred.

In: Nature Communications, Vol. 10, No. 1, 673, 08.02.2019.

Research output: Contribution to journal › Article › peer-review

Harvard

Belykh, VV, Yakovlev, DR, Glazov, MM, Grigoryev, PS, Hussain, M, Rautert, J, Dirin, DN, Kovalenko, MV & Bayer, M 2019, 'Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals', Nature Communications, vol. 10, no. 1, 673. https://doi.org/10.1038/s41467-019-08625-z

APA

Belykh, V. V., Yakovlev, D. R., Glazov, M. M., Grigoryev, P. S., Hussain, M., Rautert, J., Dirin, D. N., Kovalenko, M. V., & Bayer, M. (2019). Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals. Nature Communications, 10(1), [673]. https://doi.org/10.1038/s41467-019-08625-z

Vancouver

Belykh VV, Yakovlev DR, Glazov MM, Grigoryev PS, Hussain M, Rautert J et al. Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals. Nature Communications. 2019 Feb 8;10(1). 673. https://doi.org/10.1038/s41467-019-08625-z

Author

Belykh, Vasilii V. ; Yakovlev, Dmitri R. ; Glazov, Mikhail M. ; Grigoryev, Philipp S. ; Hussain, Mujtaba ; Rautert, Janina ; Dirin, Dmitry N. ; Kovalenko, Maksym V. ; Bayer, Manfred. / Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals. In: Nature Communications. 2019 ; Vol. 10, No. 1.

BibTeX

@article{2730d057831c4ee0b5af6176187a089d,
title = "Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals",
abstract = " The lead halide perovskites demonstrate huge potential for optoelectronic applications, high energy radiation detectors, light emitting devices and solar energy harvesting. Those materials exhibit strong spin-orbit coupling enabling efficient optical orientation of carrier spins in perovskite-based devices with performance controlled by a magnetic field. Here we show that elaborated time-resolved spectroscopy involving strong magnetic fields can be successfully used for perovskites. We perform a comprehensive study of high-quality lead halide perovskite CsPbBr 3 crystals by measuring the exciton and charge carrier g-factors, spin relaxation times and hyperfine interaction of carrier and nuclear spins by means of coherent spin dynamics. Owing to their {\textquoteleft}inverted{\textquoteright} band structure, perovskites represent appealing model systems for semiconductor spintronics exploiting the valence band hole spins, while in conventional semiconductors the conduction band electrons are considered for spin functionality. ",
keywords = "NANOCRYSTALS, EXCITONS, RASHBA",
author = "Belykh, {Vasilii V.} and Yakovlev, {Dmitri R.} and Glazov, {Mikhail M.} and Grigoryev, {Philipp S.} and Mujtaba Hussain and Janina Rautert and Dirin, {Dmitry N.} and Kovalenko, {Maksym V.} and Manfred Bayer",
year = "2019",
month = feb,
day = "8",
doi = "10.1038/s41467-019-08625-z",
language = "English",
volume = "10",
journal = "Nature Communications",
issn = "2041-1723",
publisher = "Nature Publishing Group",
number = "1",

}

RIS

TY - JOUR

T1 - Coherent spin dynamics of electrons and holes in CsPbBr 3 perovskite crystals

AU - Belykh, Vasilii V.

AU - Yakovlev, Dmitri R.

AU - Glazov, Mikhail M.

AU - Grigoryev, Philipp S.

AU - Hussain, Mujtaba

AU - Rautert, Janina

AU - Dirin, Dmitry N.

AU - Kovalenko, Maksym V.

AU - Bayer, Manfred

PY - 2019/2/8

Y1 - 2019/2/8

N2 - The lead halide perovskites demonstrate huge potential for optoelectronic applications, high energy radiation detectors, light emitting devices and solar energy harvesting. Those materials exhibit strong spin-orbit coupling enabling efficient optical orientation of carrier spins in perovskite-based devices with performance controlled by a magnetic field. Here we show that elaborated time-resolved spectroscopy involving strong magnetic fields can be successfully used for perovskites. We perform a comprehensive study of high-quality lead halide perovskite CsPbBr 3 crystals by measuring the exciton and charge carrier g-factors, spin relaxation times and hyperfine interaction of carrier and nuclear spins by means of coherent spin dynamics. Owing to their ‘inverted’ band structure, perovskites represent appealing model systems for semiconductor spintronics exploiting the valence band hole spins, while in conventional semiconductors the conduction band electrons are considered for spin functionality.

AB - The lead halide perovskites demonstrate huge potential for optoelectronic applications, high energy radiation detectors, light emitting devices and solar energy harvesting. Those materials exhibit strong spin-orbit coupling enabling efficient optical orientation of carrier spins in perovskite-based devices with performance controlled by a magnetic field. Here we show that elaborated time-resolved spectroscopy involving strong magnetic fields can be successfully used for perovskites. We perform a comprehensive study of high-quality lead halide perovskite CsPbBr 3 crystals by measuring the exciton and charge carrier g-factors, spin relaxation times and hyperfine interaction of carrier and nuclear spins by means of coherent spin dynamics. Owing to their ‘inverted’ band structure, perovskites represent appealing model systems for semiconductor spintronics exploiting the valence band hole spins, while in conventional semiconductors the conduction band electrons are considered for spin functionality.

KW - NANOCRYSTALS

KW - EXCITONS

KW - RASHBA

UR - http://www.scopus.com/inward/record.url?scp=85061224533&partnerID=8YFLogxK

UR - http://www.mendeley.com/research/coherent-spin-dynamics-electrons-holes-cspbbr-3-perovskite-crystals

U2 - 10.1038/s41467-019-08625-z

DO - 10.1038/s41467-019-08625-z

M3 - Article

C2 - 30737402

AN - SCOPUS:85061224533

VL - 10

JO - Nature Communications

JF - Nature Communications

SN - 2041-1723

IS - 1

M1 - 673

ER -

ID: 39411829