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Anomalous dependence of ionization probability and electron angular distributions on orientation of molecular axis in photoionization of H-2(+) : effect of two-center interference. / Krapivin, Dmitry A.; Telnov, Dmitry A.

In: Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 54, No. 20, 205601, 29.10.2021.

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@article{f7c92420a77d4857b3992184fc49a50f,
title = "Anomalous dependence of ionization probability and electron angular distributions on orientation of molecular axis in photoionization of H-2(+): effect of two-center interference",
abstract = "A theoretical and computational study of photoionization of the one-electron molecular ion H-2(+) initially in the 1 sigma(u) state is performed. The laser pulse is linearly polarized with the carrier wavelength in the extreme ultraviolet and soft x-ray regions. The electron wave function is obtained by solving the time-dependent Schrodinger equation with the help of the generalized pseudospectral method. The dependence of the total ionization probability and photoelectron spectra on the orientation of the molecular axis is analyzed. Within the wavelength interval 6 to 23 nm, anomalous behavior of the ionization probability is found, where it increases with the angle between the polarization vector of the external field and the molecular axis and reaches a maximum at the perpendicular orientation of the molecule. The phenomenon is explained as resulting from the two-center interference in the wave function of the emitted electron.",
keywords = "photoionization, photoelectron distributions, diatomic molecules, orientation of molecular axis, two-center interference, CONTINUUM, DYNAMICS",
author = "Krapivin, {Dmitry A.} and Telnov, {Dmitry A.}",
year = "2021",
month = oct,
day = "29",
doi = "10.1088/1361-6455/ac34de",
language = "English",
volume = "54",
journal = "Journal of the European Optical Society Part B: Quantum Optics",
issn = "0953-4075",
publisher = "IOP Publishing Ltd.",
number = "20",

}

RIS

TY - JOUR

T1 - Anomalous dependence of ionization probability and electron angular distributions on orientation of molecular axis in photoionization of H-2(+)

T2 - effect of two-center interference

AU - Krapivin, Dmitry A.

AU - Telnov, Dmitry A.

PY - 2021/10/29

Y1 - 2021/10/29

N2 - A theoretical and computational study of photoionization of the one-electron molecular ion H-2(+) initially in the 1 sigma(u) state is performed. The laser pulse is linearly polarized with the carrier wavelength in the extreme ultraviolet and soft x-ray regions. The electron wave function is obtained by solving the time-dependent Schrodinger equation with the help of the generalized pseudospectral method. The dependence of the total ionization probability and photoelectron spectra on the orientation of the molecular axis is analyzed. Within the wavelength interval 6 to 23 nm, anomalous behavior of the ionization probability is found, where it increases with the angle between the polarization vector of the external field and the molecular axis and reaches a maximum at the perpendicular orientation of the molecule. The phenomenon is explained as resulting from the two-center interference in the wave function of the emitted electron.

AB - A theoretical and computational study of photoionization of the one-electron molecular ion H-2(+) initially in the 1 sigma(u) state is performed. The laser pulse is linearly polarized with the carrier wavelength in the extreme ultraviolet and soft x-ray regions. The electron wave function is obtained by solving the time-dependent Schrodinger equation with the help of the generalized pseudospectral method. The dependence of the total ionization probability and photoelectron spectra on the orientation of the molecular axis is analyzed. Within the wavelength interval 6 to 23 nm, anomalous behavior of the ionization probability is found, where it increases with the angle between the polarization vector of the external field and the molecular axis and reaches a maximum at the perpendicular orientation of the molecule. The phenomenon is explained as resulting from the two-center interference in the wave function of the emitted electron.

KW - photoionization

KW - photoelectron distributions

KW - diatomic molecules

KW - orientation of molecular axis

KW - two-center interference

KW - CONTINUUM

KW - DYNAMICS

UR - https://www.mendeley.com/catalogue/9746024b-b3a7-360a-a65d-f208fa246c5e/

U2 - 10.1088/1361-6455/ac34de

DO - 10.1088/1361-6455/ac34de

M3 - Article

VL - 54

JO - Journal of the European Optical Society Part B: Quantum Optics

JF - Journal of the European Optical Society Part B: Quantum Optics

SN - 0953-4075

IS - 20

M1 - 205601

ER -

ID: 87640433