Research output: Contribution to journal › Article › peer-review
Anomalous dependence of ionization probability and electron angular distributions on orientation of molecular axis in photoionization of H-2(+) : effect of two-center interference. / Krapivin, Dmitry A.; Telnov, Dmitry A.
In: Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 54, No. 20, 205601, 29.10.2021.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - Anomalous dependence of ionization probability and electron angular distributions on orientation of molecular axis in photoionization of H-2(+)
T2 - effect of two-center interference
AU - Krapivin, Dmitry A.
AU - Telnov, Dmitry A.
PY - 2021/10/29
Y1 - 2021/10/29
N2 - A theoretical and computational study of photoionization of the one-electron molecular ion H-2(+) initially in the 1 sigma(u) state is performed. The laser pulse is linearly polarized with the carrier wavelength in the extreme ultraviolet and soft x-ray regions. The electron wave function is obtained by solving the time-dependent Schrodinger equation with the help of the generalized pseudospectral method. The dependence of the total ionization probability and photoelectron spectra on the orientation of the molecular axis is analyzed. Within the wavelength interval 6 to 23 nm, anomalous behavior of the ionization probability is found, where it increases with the angle between the polarization vector of the external field and the molecular axis and reaches a maximum at the perpendicular orientation of the molecule. The phenomenon is explained as resulting from the two-center interference in the wave function of the emitted electron.
AB - A theoretical and computational study of photoionization of the one-electron molecular ion H-2(+) initially in the 1 sigma(u) state is performed. The laser pulse is linearly polarized with the carrier wavelength in the extreme ultraviolet and soft x-ray regions. The electron wave function is obtained by solving the time-dependent Schrodinger equation with the help of the generalized pseudospectral method. The dependence of the total ionization probability and photoelectron spectra on the orientation of the molecular axis is analyzed. Within the wavelength interval 6 to 23 nm, anomalous behavior of the ionization probability is found, where it increases with the angle between the polarization vector of the external field and the molecular axis and reaches a maximum at the perpendicular orientation of the molecule. The phenomenon is explained as resulting from the two-center interference in the wave function of the emitted electron.
KW - photoionization
KW - photoelectron distributions
KW - diatomic molecules
KW - orientation of molecular axis
KW - two-center interference
KW - CONTINUUM
KW - DYNAMICS
UR - https://www.mendeley.com/catalogue/9746024b-b3a7-360a-a65d-f208fa246c5e/
U2 - 10.1088/1361-6455/ac34de
DO - 10.1088/1361-6455/ac34de
M3 - Article
VL - 54
JO - Journal of the European Optical Society Part B: Quantum Optics
JF - Journal of the European Optical Society Part B: Quantum Optics
SN - 0953-4075
IS - 20
M1 - 205601
ER -
ID: 87640433