Research output: Contribution to journal › Article › peer-review
A perturbed parameter model ensemble to investigate Mt. Pinatubo's 1991 initial sulfur mass emission. / Sheng, J. -X.; Weisenstein, D. K.; Luo, B. -P.; Rozanov, E.; Arfeuille, F.; Peter, T.
In: Atmospheric Chemistry and Physics, Vol. 15, No. 20, 2015, p. 11501-11512.Research output: Contribution to journal › Article › peer-review
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TY - JOUR
T1 - A perturbed parameter model ensemble to investigate Mt. Pinatubo's 1991 initial sulfur mass emission
AU - Sheng, J. -X.
AU - Weisenstein, D. K.
AU - Luo, B. -P.
AU - Rozanov, E.
AU - Arfeuille, F.
AU - Peter, T.
PY - 2015
Y1 - 2015
N2 - We have performed more than 300 atmospheric simulations of the 1991 Pinatubo eruption using the AER 2-D sulfate aerosol model to optimize the initial sulfur mass injection as a function of altitude, which in previous modeling studies has often been chosen in an ad hoc manner (e.g., by applying a rectangular-shaped emission profile). Our simulations are generated by varying a four-parameter vertical mass distribution, which is determined by a total injection mass and a skew-normal distribution function. Our results suggest that (a) the initial mass loading of the Pinatubo eruption is approximately 14 Mt of SO2; (b) the injection vertical distribution is strongly skewed towards the lower stratosphere, leading to a peak mass sulfur injection at 18-21 km; (c) the injection magnitude and height affect early southward transport of the volcanic clouds as observed by SAGE II.
AB - We have performed more than 300 atmospheric simulations of the 1991 Pinatubo eruption using the AER 2-D sulfate aerosol model to optimize the initial sulfur mass injection as a function of altitude, which in previous modeling studies has often been chosen in an ad hoc manner (e.g., by applying a rectangular-shaped emission profile). Our simulations are generated by varying a four-parameter vertical mass distribution, which is determined by a total injection mass and a skew-normal distribution function. Our results suggest that (a) the initial mass loading of the Pinatubo eruption is approximately 14 Mt of SO2; (b) the injection vertical distribution is strongly skewed towards the lower stratosphere, leading to a peak mass sulfur injection at 18-21 km; (c) the injection magnitude and height affect early southward transport of the volcanic clouds as observed by SAGE II.
KW - LARGE VOLCANIC-ERUPTIONS
KW - STRATOSPHERIC AEROSOL
KW - CLIMATE MODEL
KW - 2-DIMENSIONAL MODEL
KW - II MEASUREMENTS
KW - SO2
KW - SIMULATIONS
KW - INSTRUMENTS
KW - EVOLUTION
KW - JUNE
U2 - 10.5194/acp-15-11501-2015
DO - 10.5194/acp-15-11501-2015
M3 - статья
VL - 15
SP - 11501
EP - 11512
JO - Atmospheric Chemistry and Physics
JF - Atmospheric Chemistry and Physics
SN - 1680-7316
IS - 20
ER -
ID: 105536688