Generalized Floquet formulation of time-dependent density functional theory for many-electron systems in intense laser fields

DA Telnov, S.-I. Chu

Результат исследований: Публикации в книгах, отчётах, сборниках, трудах конференцийстатья в сборнике материалов конференциинаучнаярецензирование

Аннотация

We present some recent new developments of the generalized Floquet formulation of time-dependent density functional theory (TDDFT) for nonperturbative treatment of multiphoton processes of many-electron quantum systems in intense monochromatic or multi-color laser fields. It is shown that the periodically or quasi-periodically (polychromatic) time-dependent Kohn-Sham equations can be exactly transformed into an equivalent time-independent Floquet Hamiltonian matrix eigenvalue problems. A procedure is presented for the treatment of bound-bound transitions. For the bound-free transitions, such as multiphoton ionization (MPI) or multiphoton dissociation processes, we introduce the notion of "complex density" and present a non-Hermitian Floquet formalism for the treatment of complex quasienergies of individual spin-orbitals and total many-electron systems. The procedure is demonstrated by a case study of photoionization of He atoms in the photon energy range of 25 to 50 eV. Good agreement with recent experimental data is obtained. We also perform some MPI study of He and Be atoms in intense monochromatic and two-color laser fields.

Язык оригиналаАнглийский
Название основной публикацииMULTIPHOTON PROCESSES
РедакторыLF DiMauro, RR Freeman, KC Kulander
ИздательAmerican Institute of Physics
Страницы304-315
Число страниц12
ISBN (печатное издание)1-56396-946-7
СостояниеОпубликовано - 2000
Событие8th International Conference on Multiphoton Processes (ICOMP VIII) - MONTEREY, Канада
Продолжительность: 3 окт 19998 окт 1999

Серия публикаций

НазваниеAIP Conference Proceedings
ИздательAMER INST PHYSICS
Том525
ISSN (печатное издание)0094-243X

конференция

конференция8th International Conference on Multiphoton Processes (ICOMP VIII)
СтранаКанада
ГородMONTEREY
Период3/10/998/10/99

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