DOI

Two-step, two-color populations of T-shaped ArI2(E,vE = 0-2,nE) complexes, accompanied by their electronic predissociation, have been studied. The luminescence spectra of the ion-pair I2(IP,vIP), IP = D′2g, β1g, D 0 u + , molecules, ArI2(E 0 g + ,vE = 0-2,nE) complexes were measured, and the branching ratios of the I2(IP,vIP) populations and ArI2(E,vE = 0-2,nE) lifetimes were determined. The comparison of the spectroscopic characteristics of ArI2(E,vE,nE) complexes obtained in this work and by Macarem and Loomis [Chem. Phys. Lett. 826, 140642 (2023)], has been carried out. Measurements of true luminescence spectra, corrected for the spectral dependence of the registration system sensitivity, allow us to determine the branching coefficients of the population of the vibrational and electronic predissociation products and even their vibrational distributions. In addition, this method allows us to determine the branching ratios of the ArI2(E,vE, n b E , n s E ) populations and lifetimes of the complex if its vibrational predissociation is impossible.
Translated title of the contributionЗаселение и распад ионно-парных состояний ван-дер-ваальсовых Т-образноых комплекса ArI2 исследованы с использованием двухступенчатого, двухцветного заселения и измерений спектров люминесценции
Original languageEnglish
Article number044306
Number of pages8
JournalJournal of Chemical Physics
Volume163
Issue number4
DOIs
StatePublished - 24 Jul 2025

ID: 140755310