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Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake. / Mikhailov, E.; Merkulov, V; Vlasenko, S.; Rose, D.; Poschl, U.

In: Atmospheric Chemistry and Physics Discussions, No. 11, 2011, p. 30877–30918.

Research output: Contribution to journal › Article › peer-review

Harvard

Mikhailov, E, Merkulov, V, Vlasenko, S, Rose, D & Poschl, U 2011, 'Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake', Atmospheric Chemistry and Physics Discussions, no. 11, pp. 30877–30918. https://doi.org/doi:10.5194/acpd-11-30877-2011

APA

Mikhailov, E., Merkulov, V., Vlasenko, S., Rose, D., & Poschl, U. (2011). Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake. Atmospheric Chemistry and Physics Discussions, (11), 30877–30918. https://doi.org/doi:10.5194/acpd-11-30877-2011

Vancouver

Mikhailov E, Merkulov V, Vlasenko S, Rose D, Poschl U. Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake. Atmospheric Chemistry and Physics Discussions. 2011;(11):30877–30918. https://doi.org/doi:10.5194/acpd-11-30877-2011

Author

Mikhailov, E. ; Merkulov, V ; Vlasenko, S. ; Rose, D. ; Poschl, U. / Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake. In: Atmospheric Chemistry and Physics Discussions. 2011 ; No. 11. pp. 30877–30918.

BibTeX

@article{5b071e5e2c0b457389df2cba0147e4ed,
title = "Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake",
abstract = "Abstract. In this study we derive and apply a mass-based hygroscopicity parameter interaction model for efficient description of concentration-dependent water uptake by atmospheric aerosol particles. The model approach builds on the single hygroscopicity parameter model of Petters and Kreidenweis (2007). We introduce an observable mass-based hygroscopicity parameter κm, which can be deconvoluted into a dilute intrinsic hygroscopicity parameter (κm,∞) and additional self- and cross-interaction parameters describing non-ideal solution behavior and concentration dependencies of single- and multi-component systems. For sodium chloride, the κm-interaction model (KIM) captures the observed concentration and humidity dependence of the hygroscopicity parameter and is in good agreement with an accurate reference model based on the Pitzer ion-interaction approach (Aerosol Inorganic Model, AIM). For atmospheric aerosol samples collected from boreal rural air and from pristine tropical rainforest air (secondary organic",
author = "E. Mikhailov and V Merkulov and S. Vlasenko and D. Rose and U. Poschl",
year = "2011",
doi = "doi:10.5194/acpd-11-30877-2011",
language = "English",
pages = "30877–30918",
journal = "Atmospheric Chemistry and Physics Discussions",
issn = "1680-7367",
publisher = "Copernicus GmbH ",
number = "11",

}

RIS

TY - JOUR

T1 - Mass-based hygroscopicity parameter interaction model and measurement of atmospheric aerosol water uptake

AU - Mikhailov, E.

AU - Merkulov, V

AU - Vlasenko, S.

AU - Rose, D.

AU - Poschl, U.

PY - 2011

Y1 - 2011

N2 - Abstract. In this study we derive and apply a mass-based hygroscopicity parameter interaction model for efficient description of concentration-dependent water uptake by atmospheric aerosol particles. The model approach builds on the single hygroscopicity parameter model of Petters and Kreidenweis (2007). We introduce an observable mass-based hygroscopicity parameter κm, which can be deconvoluted into a dilute intrinsic hygroscopicity parameter (κm,∞) and additional self- and cross-interaction parameters describing non-ideal solution behavior and concentration dependencies of single- and multi-component systems. For sodium chloride, the κm-interaction model (KIM) captures the observed concentration and humidity dependence of the hygroscopicity parameter and is in good agreement with an accurate reference model based on the Pitzer ion-interaction approach (Aerosol Inorganic Model, AIM). For atmospheric aerosol samples collected from boreal rural air and from pristine tropical rainforest air (secondary organic

AB - Abstract. In this study we derive and apply a mass-based hygroscopicity parameter interaction model for efficient description of concentration-dependent water uptake by atmospheric aerosol particles. The model approach builds on the single hygroscopicity parameter model of Petters and Kreidenweis (2007). We introduce an observable mass-based hygroscopicity parameter κm, which can be deconvoluted into a dilute intrinsic hygroscopicity parameter (κm,∞) and additional self- and cross-interaction parameters describing non-ideal solution behavior and concentration dependencies of single- and multi-component systems. For sodium chloride, the κm-interaction model (KIM) captures the observed concentration and humidity dependence of the hygroscopicity parameter and is in good agreement with an accurate reference model based on the Pitzer ion-interaction approach (Aerosol Inorganic Model, AIM). For atmospheric aerosol samples collected from boreal rural air and from pristine tropical rainforest air (secondary organic

U2 - doi:10.5194/acpd-11-30877-2011

DO - doi:10.5194/acpd-11-30877-2011

M3 - Article

SP - 30877

EP - 30918

JO - Atmospheric Chemistry and Physics Discussions

JF - Atmospheric Chemistry and Physics Discussions

SN - 1680-7367

IS - 11

ER -

ID: 5254255