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Electric field assisted alignment of monoatomic carbon chains. / Kutrovskaya, Stella; Chestnov, Igor; Osipov, Anton; Samyshkin, Vlad; Sapegina, Irina; Kavokin, Alexey; Kucherik, Alexey.

In: Scientific Reports, Vol. 10, No. 1, 9709, 16.06.2020.

Research output: Contribution to journal › Article › peer-review

Harvard

Kutrovskaya, S, Chestnov, I, Osipov, A, Samyshkin, V, Sapegina, I, Kavokin, A & Kucherik, A 2020, 'Electric field assisted alignment of monoatomic carbon chains', Scientific Reports, vol. 10, no. 1, 9709. https://doi.org/10.1038/s41598-020-65356-8

APA

Kutrovskaya, S., Chestnov, I., Osipov, A., Samyshkin, V., Sapegina, I., Kavokin, A., & Kucherik, A. (2020). Electric field assisted alignment of monoatomic carbon chains. Scientific Reports, 10(1), [9709]. https://doi.org/10.1038/s41598-020-65356-8

Vancouver

Kutrovskaya S, Chestnov I, Osipov A, Samyshkin V, Sapegina I, Kavokin A et al. Electric field assisted alignment of monoatomic carbon chains. Scientific Reports. 2020 Jun 16;10(1). 9709. https://doi.org/10.1038/s41598-020-65356-8

Author

Kutrovskaya, Stella ; Chestnov, Igor ; Osipov, Anton ; Samyshkin, Vlad ; Sapegina, Irina ; Kavokin, Alexey ; Kucherik, Alexey. / Electric field assisted alignment of monoatomic carbon chains. In: Scientific Reports. 2020 ; Vol. 10, No. 1.

BibTeX

@article{5692fbd335eb446a866bee740fd65891,
title = "Electric field assisted alignment of monoatomic carbon chains",
abstract = "We stabilize monoatomic carbon chains in water by attaching them to gold nanoparticles (NPs) by means of the laser ablation process. Resulting nanoobjects represent pairs of NPs connected by multiple straight carbon chains of several nanometer lengths. If NPs at the opposite ends of a chain differ in size, the structure acquires a dipole moment due to the difference in work functions of the two NPs. We take advantage of the dipole polarisation of carbon chains for ordering them by the external electric field. We deposit them on a glass substrate by the sputtering method in the presence of static electric fields of magnitudes up to 105 V/m. The formation of one-dimensional carbyne quasi-crystals deposited on a substrate is evidenced by high-resolution TEM and X-ray diffraction measurements. The original kinetic model describing the dynamics of ballistically flowing nano-dipoles reproduces the experimental diagram of orientation of the deposited chains.",
keywords = "FERMI-LEVEL EQUILIBRATION, LASER-INDUCED SYNTHESIS, WORK FUNCTION, CARBYNE, POTENTIALS, TRANSPORT",
author = "Stella Kutrovskaya and Igor Chestnov and Anton Osipov and Vlad Samyshkin and Irina Sapegina and Alexey Kavokin and Alexey Kucherik",
year = "2020",
month = jun,
day = "16",
doi = "10.1038/s41598-020-65356-8",
language = "English",
volume = "10",
journal = "Scientific Reports",
issn = "2045-2322",
publisher = "Nature Publishing Group",
number = "1",

}

RIS

TY - JOUR

T1 - Electric field assisted alignment of monoatomic carbon chains

AU - Kutrovskaya, Stella

AU - Chestnov, Igor

AU - Osipov, Anton

AU - Samyshkin, Vlad

AU - Sapegina, Irina

AU - Kavokin, Alexey

AU - Kucherik, Alexey

PY - 2020/6/16

Y1 - 2020/6/16

N2 - We stabilize monoatomic carbon chains in water by attaching them to gold nanoparticles (NPs) by means of the laser ablation process. Resulting nanoobjects represent pairs of NPs connected by multiple straight carbon chains of several nanometer lengths. If NPs at the opposite ends of a chain differ in size, the structure acquires a dipole moment due to the difference in work functions of the two NPs. We take advantage of the dipole polarisation of carbon chains for ordering them by the external electric field. We deposit them on a glass substrate by the sputtering method in the presence of static electric fields of magnitudes up to 105 V/m. The formation of one-dimensional carbyne quasi-crystals deposited on a substrate is evidenced by high-resolution TEM and X-ray diffraction measurements. The original kinetic model describing the dynamics of ballistically flowing nano-dipoles reproduces the experimental diagram of orientation of the deposited chains.

AB - We stabilize monoatomic carbon chains in water by attaching them to gold nanoparticles (NPs) by means of the laser ablation process. Resulting nanoobjects represent pairs of NPs connected by multiple straight carbon chains of several nanometer lengths. If NPs at the opposite ends of a chain differ in size, the structure acquires a dipole moment due to the difference in work functions of the two NPs. We take advantage of the dipole polarisation of carbon chains for ordering them by the external electric field. We deposit them on a glass substrate by the sputtering method in the presence of static electric fields of magnitudes up to 105 V/m. The formation of one-dimensional carbyne quasi-crystals deposited on a substrate is evidenced by high-resolution TEM and X-ray diffraction measurements. The original kinetic model describing the dynamics of ballistically flowing nano-dipoles reproduces the experimental diagram of orientation of the deposited chains.

KW - FERMI-LEVEL EQUILIBRATION

KW - LASER-INDUCED SYNTHESIS

KW - WORK FUNCTION

KW - CARBYNE

KW - POTENTIALS

KW - TRANSPORT

UR - http://www.scopus.com/inward/record.url?scp=85086668258&partnerID=8YFLogxK

UR - https://www.mendeley.com/catalogue/64a11fcc-6c1c-314b-a99d-14ac8d9c2f8e/

U2 - 10.1038/s41598-020-65356-8

DO - 10.1038/s41598-020-65356-8

M3 - Article

C2 - 32546798

AN - SCOPUS:85086668258

VL - 10

JO - Scientific Reports

JF - Scientific Reports

SN - 2045-2322

IS - 1

M1 - 9709

ER -

ID: 62025546